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透气、自粘干电极,可在运动过程中稳定监测生理电信号。

Breathable, Self-Adhesive Dry Electrodes for Stable Electrophysiological Signal Monitoring During Exercise.

机构信息

The State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Science, Shanghai 200050, China.

University of Chinese Academy of Sciences, 19 Yuquan Road, Beijing 100049, China.

出版信息

ACS Appl Mater Interfaces. 2022 Mar 16;14(10):12812-12823. doi: 10.1021/acsami.1c23322. Epub 2022 Mar 2.

Abstract

On-skin electrodes with high air permeability, low thickness, low elastic modulus, and high adhesion are essential for biomedical signal recordings, which provide data for sports management and biomedical applications. However, nanothickness electrodes interacting with the skin by van der Waals force can be interfered with by sweating, and elastomers with high adhesion prepared by modification are not satisfactory in terms of air permeability. Here, a dry electrode with high stretchability (598%), low elastic modulus (5 MPa), high air permeability (726 g m d), and high adhesion (6.33 kPa) was fabricated by semi-embedding Ag nanowires into nonyl and glycerol-modified polyvinyl alcohol. Furthermore, a small amount of 40 wt % ethanol was sprayed on the skin to facilitate microdissolution of the substrate and form immediate conformability with skin texture. The dry electrodes can record high-quality electrocardiogram and electromyogram signals through a robust contact with the skin under skin deformation, with a water stream, or after running for 1 h. The film can also be served as the substrate for self-adhesive strain sensors to monitor motion with higher quality than nonadhesive polydimethylsilane-based sensors.

摘要

具有高透气性、低厚度、低弹性模量和高附着力的皮肤贴合电极对于生物医学信号记录至关重要,这些信号记录为运动管理和生物医学应用提供了数据。然而,通过范德华力与皮肤相互作用的纳米厚度电极可能会受到出汗的干扰,而通过修饰制备的具有高附着力的弹性体在透气性方面并不理想。在这里,通过将银纳米线半嵌入壬基和甘油改性的聚乙烯醇中,制备了一种具有高拉伸性(598%)、低弹性模量(5 MPa)、高透气性(726 g m d)和高附着力(6.33 kPa)的干电极。此外,只需在皮肤上喷洒少量 40wt%乙醇,就可以促进基底的微溶解,并立即与皮肤纹理形成贴合。该干电极可以在皮肤变形、水流或跑步 1 小时后通过与皮肤的牢固接触记录高质量的心电图和肌电图信号。该薄膜还可用作自粘性应变传感器的基底,以比非粘性基于聚二甲基硅氧烷的传感器更高的质量来监测运动。

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