De Leo Eva, Rossinelli Aurelio A, Marqués-Gallego Patricia, Poulikakos Lisa V, Norris David J, Prins Ferry
Optical Materials Engineering Laboratory, ETH Zürich, Leonhardstrasse 21, Zürich 8092, Switzerland.
Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, Calle Francisco Tomas y Valiente 6, Madrid 29049, Spain.
Nanoscale. 2022 Mar 31;14(13):4929-4934. doi: 10.1039/d1nr07136j.
Colloidal quantum-dots (cQDs) are finding increasingly widespread application in photonics and optoelectronics, providing high brightness and record-wide colour gamuts. However, the external quantum efficiencies in thin-film device architectures are still limited due to losses into waveguide modes and different strategies are being explored to promote the outcoupling of emission. Here we use a template-stripping-based direct-patterning strategy to fabricate linear gratings at the surface of cQD thin films. The linear gratings enhance optical outcoupling through Bragg scattering, yielding bright emission with a strong degree of linear polarization. By patterning linear gratings with different periodicities and orientations onto a film of mixed-colour cQDs, we demonstrate polarization-based active colour tuning of the thin-film emission.
胶体量子点(cQDs)在光子学和光电子学中的应用越来越广泛,具有高亮度和创纪录的宽色域。然而,由于进入波导模式的损耗,薄膜器件结构中的外量子效率仍然有限,人们正在探索不同的策略来促进发射光的外耦合。在这里,我们使用基于模板剥离的直接图案化策略在cQD薄膜表面制造线性光栅。线性光栅通过布拉格散射增强光外耦合,产生具有强线性偏振度的明亮发射。通过在混合颜色的cQD薄膜上图案化具有不同周期和取向的线性光栅,我们展示了基于偏振的薄膜发射有源颜色调谐。