Coghlan Jill, Benet Alexander, Kumaran Preethi, Ford Michael, Veale Lawrie, Skilton St John, Saveliev Sergei, Schwendeman Anna A
Department of Pharmaceutical Sciences, College of Pharmacy, University of Michigan, Ann Arbor, MI, United States.
MS Bioworks, Ann Arbor, MI, United States.
Front Bioeng Biotechnol. 2022 Mar 14;10:862456. doi: 10.3389/fbioe.2022.862456. eCollection 2022.
Post translational modifications (PTMs) have been shown to negatively impact protein efficacy and safety by altering its native conformation, stability, target binding and/or pharmacokinetics. One PTM in particular, shuffled disulfide bonds, has been linked to decreased potency and increased immunogenicity of protein therapeutics. In an effort to gain more insights into the effects of shuffled disulfide bonds on protein therapeutics' safety and efficacy, we designed and further optimized a semi-automated LC-MS/MS method for disulfide bond characterization on two IgG1 protein therapeutics-rituximab and bevacizumab. We also compared originator vs. biosimilar versions of the two therapeutics to determine if there were notable variations in the disulfide shuffling and overall degradation between originator and biosimilar drug products. From our resulting data, we noticed differences in how the two proteins degraded. Bevacizumab had a general upward trend in shuffled disulfide bond levels over the course of a 4-week incubation (0.58 ± 0.08% to 1.46 ± 1.10% for originator) whereas rituximab maintained similar levels throughout the incubation (0.24 ± 0.21% to 0.51 ± 0.11% for originator). When we measured degradation by SEC and SDS-PAGE, we observed trends that correlated with the LC-MS/MS data. Across all methods, we observed that the originator and biosimilar drugs performed similarly. The results from this study will help provide groundwork for comparative disulfide shuffling analysis by LC-MS/MS and standard analytical methodology implementation for the development and regulatory approval of biosimilars.
翻译后修饰(PTMs)已被证明会通过改变蛋白质的天然构象、稳定性、靶点结合和/或药代动力学,对蛋白质的疗效和安全性产生负面影响。特别是一种翻译后修饰,即重排二硫键,已被证明与蛋白质治疗药物的效力降低和免疫原性增加有关。为了更深入了解重排二硫键对蛋白质治疗药物安全性和疗效的影响,我们设计并进一步优化了一种半自动液相色谱-串联质谱(LC-MS/MS)方法,用于对两种IgG1蛋白质治疗药物——利妥昔单抗和贝伐单抗的二硫键进行表征。我们还比较了这两种治疗药物的原研药和生物类似药版本,以确定原研药和生物类似药产品在二硫键重排和整体降解方面是否存在显著差异。从我们得到的数据中,我们注意到这两种蛋白质降解方式的差异。在4周的孵育过程中,贝伐单抗的重排二硫键水平总体呈上升趋势(原研药从0.58±0.08%升至1.46±1.10%),而利妥昔单抗在整个孵育过程中保持相似水平(原研药从0.24±0.21%升至0.51±0.11%)。当我们通过尺寸排阻色谱(SEC)和十二烷基硫酸钠聚丙烯酰胺凝胶电泳(SDS-PAGE)测量降解时,我们观察到与LC-MS/MS数据相关的趋势。在所有方法中,我们观察到原研药和生物类似药的表现相似。这项研究的结果将有助于为通过LC-MS/MS进行比较二硫键重排分析以及为生物类似药的开发和监管批准实施标准分析方法奠定基础。