Department of Chemistry, McGill University, Montréal, QC, H3A 2K6, Canada.
Department of Atmospheric & Oceanic Sciences, McGill University, Montréal, QC, H3A 2K6, Canada.
Environ Sci Pollut Res Int. 2022 Aug;29(38):58133-58148. doi: 10.1007/s11356-022-19708-8. Epub 2022 Apr 1.
Airports are identified hotspots for air pollution, notably for fine particles (PM) that are pivotal in aerosol-cloud interaction processes of climate change and human health. We herein studied the field observation and statistical analysis of 10-year data of PM and selected emitted co-pollutants (CO, NO, and O), in the vicinity of three major Canadian airports, with moderate to cold climates. The decadal data analysis indicated that in colder climate airports, pollutants like PM and CO accumulate disproportionally to their emissions in fall and winter, in comparison to airports in milder climates. Decadal daily averages and standard errors of PM concentrations were as follows: Vancouver, 5.31 ± 0.017; Toronto, 6.71 ± 0.199; and Montreal, 7.52 ± 0.023 μg/m. The smallest and the coldest airport with the least flights/passengers had the highest PM concentration. QQQ-ICP-MS/MS and HR-S/TEM analysis of aerosols near Montreal Airport indicated a wide range of emerging contaminants (Cd, Mo, Co, As, Ni, Cr, and Pb) ranging from 0.90 to 622 μg/L, which were also observed in the atmosphere. During the lockdown, a pronounced decrease in the concentrations of PM and submicron particles, including nanoparticles in residential areas close to airports was observed, conforming with the recommended workplace health thresholds (~ 2 × 10 cm), while before the lockdown, condensable particles were up to ~ 1 × 10 cm. Targeted reduction of PM emission is recommended for cold climate regions.
机场被认为是空气污染的热点区域,尤其是对细颗粒物(PM)而言,这些细颗粒物在气候变化和人类健康的气溶胶-云相互作用过程中起着关键作用。本研究对加拿大三个主要机场附近 10 年的 PM 及选定的排放污染物(CO、NO 和 O)的现场观测和统计分析数据进行了研究,这些机场所处地区的气候属于中等到寒冷气候。十年数据分析表明,在气候较冷的机场,污染物如 PM 和 CO 的积累量与其在秋季和冬季的排放量不成比例,而气候较温和的机场则不是这样。 PM 浓度的十年日平均值和标准误差如下:温哥华为 5.31±0.017μg/m3;多伦多为 6.71±0.199μg/m3;蒙特利尔为 7.52±0.023μg/m3。航班/乘客数量最少且气候最冷的机场 PM 浓度最高。蒙特利尔机场附近气溶胶的 QQQ-ICP-MS/MS 和 HR-S/TEM 分析表明,存在范围广泛的新兴污染物(Cd、Mo、Co、As、Ni、Cr 和 Pb),浓度在 0.90 至 622μg/L 之间,这些污染物也存在于大气中。在封锁期间,靠近机场的居民区中 PM 和亚微米颗粒(包括纳米颗粒)的浓度明显下降,符合推荐的工作场所健康阈值(约 2×10cm),而在封锁之前,可凝结颗粒的浓度高达约 1×10cm。建议在寒冷气候地区减少 PM 排放。