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Sr[化学式:见原文]Ca[化学式:见原文]Co[化学式:见原文]P[化学式:见原文]中的压力驱动磁有序

Pressure driven magnetic order in Sr[Formula: see text]Ca[Formula: see text]Co[Formula: see text]P[Formula: see text].

作者信息

Forslund Ola Kenji, Andreica Daniel, Sassa Yasmine, Imai Masaki, Michioka Chishiro, Yoshimura Kazuyoshi, Guguchia Zurab, Shermadini Zurab, Khasanov Rustem, Sugiyama Jun, Månsson Martin

机构信息

Department of Applied Physics, KTH Royal Institute of Technology, 106 91 Stockholm, Sweden.

Faculty of Physics, Babes-Bolyai University, 400084 Cluj-Napoca, Romania.

出版信息

Sci Rep. 2022 Oct 20;12(1):17526. doi: 10.1038/s41598-022-21699-y.

Abstract

The magnetic phase diagram of Sr[Formula: see text]Ca[Formula: see text]Co[Formula: see text]P[Formula: see text] as a function of hydrostatic pressure and temperature is investigated by means of high pressure muon spin rotation, relaxation and resonance ([Formula: see text]SR). The weak pressure dependence for the [Formula: see text] compounds suggests that the rich phase diagram of Sr[Formula: see text]Ca[Formula: see text]Co[Formula: see text]P[Formula: see text] as a function of x at ambient pressure may not solely be attributed to chemical pressure effects. The [Formula: see text] compound on the other hand reveals a high pressure dependence, where the long range magnetic order is fully suppressed at [Formula: see text] kbar, which seem to be a first order transition. In addition, an intermediate phase consisting of magnetic domains is formed above [Formula: see text] kbar where they co-exist with a magnetically disordered state. These domains are likely to be ferromagnetic islands (FMI) and consist of an high- (FMI-[Formula: see text]) and low-temperature (FMI-[Formula: see text]) region, respectively, separated by a phase boundary at [Formula: see text] K. This kind of co-existence is unusual and is originating from a coupling between lattice and magnetic degrees of freedoms.

摘要

通过高压μ子自旋旋转、弛豫和共振(μSR)研究了Sr[化学式:见原文]Ca[化学式:见原文]Co[化学式:见原文]P[化学式:见原文]的磁相图随静水压力和温度的变化。对于[化学式:见原文]化合物,其对压力的微弱依赖性表明,在常压下Sr[化学式:见原文]Ca[化学式:见原文]Co[化学式:见原文]P[化学式:见原文]随x变化的丰富相图可能不能仅仅归因于化学压力效应。另一方面,[化学式:见原文]化合物显示出对高压的依赖性,在[压力值:见原文]千巴时,长程磁有序被完全抑制,这似乎是一个一级转变。此外,在[压力值:见原文]千巴以上形成了一个由磁畴组成的中间相,在那里它们与磁无序状态共存。这些畴可能是铁磁岛(FMI),分别由一个高温(FMI-[温度值:见原文])和低温(FMI-[温度值:见原文])区域组成,在[温度值:见原文]K处由一个相界分隔。这种共存情况不寻常,是由晶格和磁自由度之间的耦合引起的。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e2c4/9585139/5f9db05b567a/41598_2022_21699_Fig1_HTML.jpg

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