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银的半衰期测定。

Half-life determination of Ag.

机构信息

Northwest Institute of Nuclear Technology, Xi'an, 710024, China.

Northwest Institute of Nuclear Technology, Xi'an, 710024, China.

出版信息

Appl Radiat Isot. 2023 Apr;194:110689. doi: 10.1016/j.apradiso.2023.110689. Epub 2023 Jan 28.

Abstract

Ag is a radionuclide that can be generated by neutron capture on Pd and whose decay properties and production feasibility make it a potential therapeutic agent against arthritis. Due to the discrepancies of recent published values of the half-life of Ag with previous published works which are not thoroughly documented for detailed experiment procedures and uncertainty budgets evaluation, an independent redetermination of the Ag half-life value is required. In this work, a solid Ag source was prepared and repeatedly measured in a high purity Germanium (HPGe) detector to determine its half-life. In total, more than fifty measurements were performed over a period of 26.3 days, corresponding to ∼3.5 half-lives of Ag. The experimental method and corresponding uncertainty budget are presented. The result of 7.419(15) days is consistent with the recently published value, 7.423(13) days, by Collins et al. and deviates by 0.418% from the currently recommended value 7.45(1) days. A new recommend half-life value of 7.437(7) days was determined utilizing all available experimental values by a power-moderated mean (PMM) method.

摘要

银是一种放射性核素,可以通过钯的中子捕获产生,其衰变性质和生产可行性使其成为治疗关节炎的潜在治疗剂。由于最近发表的银半衰期值与以前发表的工作存在差异,这些工作没有详细记录实验过程和不确定度预算的评估,因此需要对银半衰期值进行独立的重新确定。在这项工作中,制备了固体银源,并在高纯锗(HPGe)探测器中反复测量,以确定其半衰期。总共进行了五十多次测量,历时 26.3 天,相当于银的约 3.5 个半衰期。介绍了实验方法和相应的不确定度预算。结果为 7.419(15)天,与 Collins 等人最近发表的 7.423(13)天的值一致,与目前推荐的 7.45(1)天的值偏差 0.418%。利用所有可用的实验值,通过幂调制平均值(PMM)方法确定了新的推荐半衰期值 7.437(7)天。

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