Wen Jiahao, Zhou Lean, Tang Qingxin, Xiao Xiaozhen, Sun Shiquan
School of Hydraulic and Environmental Engineering, Changsha University of Science & Technology, Changsha 410114, China; Key Laboratory of Dongting Lake Aquatic Eco-Environmental Control and Restoration of Hunan Province, Changsha 410114, China.
School of Hydraulic and Environmental Engineering, Changsha University of Science & Technology, Changsha 410114, China; Key Laboratory of Dongting Lake Aquatic Eco-Environmental Control and Restoration of Hunan Province, Changsha 410114, China.
Ecotoxicol Environ Saf. 2023 Jun 14;262:115133. doi: 10.1016/j.ecoenv.2023.115133.
Graphitic carbon nitride (g-CN) has received much attention due to its unique characteristics of stable physicochemical features, facile preparation, and inexpensive cost. However, the bulk g-CN has a weak capacity for pollutant degradation and needs to be modified for real application. Therefore, extensive research has been done on g-CN, and the discovery of the novel zero-dimensional nanomaterials known as carbon quantum dots (CQDs) provided it with a unique modification option. In this review, the development for the removal of organic pollutants by g-CN/CQDs was discussed. Firstly, the preparation of g-CN/CQDs were introduced. Then, the application and the degradation mechanism of g-CN/CQDs were briefly described. And the discussion of the influencing factors on g-CN/CQDs' ability to degrade organic pollutants came in third. Finally, the conclusions of photocatalytic degradation of organic pollutants by g-CN/CQDs and future perspectives followed. This review will strengthen the understanding of the photocatalytic degradation of real organic wastewater by g-CN/CQDs, including their preparation, application, mechanism, and influencing factors.
石墨相氮化碳(g-CN)因其具有稳定的物理化学特性、制备简便且成本低廉等独特性质而备受关注。然而,块状g-CN对污染物的降解能力较弱,需要进行改性才能实际应用。因此,人们对g-CN开展了广泛研究,而新型零维纳米材料碳量子点(CQDs)的发现为其提供了一种独特的改性选择。在这篇综述中,探讨了g-CN/CQDs去除有机污染物的研究进展。首先,介绍了g-CN/CQDs的制备方法。然后,简要描述了g-CN/CQDs的应用及降解机理。第三部分讨论了影响g-CN/CQDs降解有机污染物能力的因素。最后是g-CN/CQDs光催化降解有机污染物的结论及未来展望。这篇综述将加深人们对g-CN/CQDs光催化降解实际有机废水的理解,包括其制备、应用、机理和影响因素。