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利用环保且经济高效的基于气凝胶的界面蒸发器和卓越的光催化能力提高太阳能驱动的水净化。

Improved solar-driven water purification using an eco-friendly and cost-effective aerogel-based interfacial evaporator with exceptional photocatalytic capabilities.

机构信息

College of Veterinary Medicine, Yangzhou University, Yangzhou, 225009, PR China.

School of Chemistry and Chemical Engineering, Yangzhou University, 180 Siwangting Road, Yangzhou, Jiangsu, 225002, PR China.

出版信息

J Environ Manage. 2024 Feb;351:119916. doi: 10.1016/j.jenvman.2023.119916. Epub 2023 Dec 26.

Abstract

As a promising solution to address the global challenge of freshwater scarcity, solar-powered interfacial steam generation has undergone notable advancements. This study introduces a novel solar-driven interfacial evaporation membrane (ZnInS@SiO/ACSA, ZSAS) comprising a ZnInS@SiO composite and a black sodium alginate aerogel infused with activated carbon. The ZSAS membrane demonstrates exceptional light absorption and thermal insulation, leading to elevated surface temperatures and reduced heat dissipation into the bulk water. Furthermore, the incorporation of AC reinforces the mechanical properties of the ZSAS membrane and enhances the water purification performance. These collective features result in an impressive evaporation rate of 1.485 kg m h and a high photothermal conversion efficiency of 91.2% under 1 sun irradiation for the optimal ZSAS membrane. Moreover, the optimal ZSAS membrane can effectively remove salts, heavy metal ions, and organic pollutants, benefitting from its superior evaporation separation effect and the photocatalytic properties of the ZnInS@SiO composite.

摘要

作为解决全球淡水短缺挑战的一种有前途的解决方案,太阳能界面蒸汽发生技术取得了显著进展。本研究介绍了一种新型的太阳能驱动界面蒸发膜(ZnInS@SiO/ACSA,ZSAS),它由 ZnInS@SiO 复合材料和一种黑色海藻酸钠气凝胶组成,其中注入了活性炭。ZSAS 膜具有优异的光吸收和隔热性能,导致表面温度升高,进入体相水的热量减少。此外,AC 的加入增强了 ZSAS 膜的机械性能,并提高了水净化性能。这些综合特性使得在 1 个太阳照射下,最佳 ZSAS 膜的蒸发速率达到 1.485kg m h,光热转换效率高达 91.2%。此外,最佳 ZSAS 膜可以有效地去除盐、重金属离子和有机污染物,这得益于其优越的蒸发分离效果和 ZnInS@SiO 复合材料的光催化性能。

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