Cho M S, Chung H-K, Foord M E, Libby S B, Cho B I
Gwangju Institute of Science and Technology, Department of Physics and Photon Science, Gwangju 61005, South Korea.
Lawrence Livermore National Laboratory, 7000 East Avenue, Livermore, California 94550, USA.
Phys Rev E. 2024 Apr;109(4-2):045207. doi: 10.1103/PhysRevE.109.045207.
The interplay of kinetic electron physics and atomic processes in ultrashort laser-plasma interactions provides a comprehensive understanding of the impact of the electron energy distribution on plasma properties. Notably, nonequilibrium electrons play a vital role in collisional ionization, influencing ionization degrees and spectra. This paper introduces a computational model that integrates the physics of kinetic electrons and atomic processes, utilizing a Boltzmann equation for nonequilibrium electrons and a collisional-radiative model for atomic state populations. The model is used to investigate the influence of nonequilibrium electrons on collisional ionization rates and its effect on the population distribution, as observed in a widely known experiment [Young et al., Nature (London) 466, 56 (2010)0028-083610.1038/nature09177]. The study reveals a significant nonequilibrium electron presence during XFEL-matter interactions, profoundly affecting collisional ionization rates in the gas plasma, thereby necessitating careful consideration of the Collisional-Radiative model applied to such systems.
在超短激光-等离子体相互作用中,动力学电子物理学与原子过程之间的相互作用为全面理解电子能量分布对等离子体特性的影响提供了依据。值得注意的是,非平衡电子在碰撞电离中起着至关重要的作用,影响着电离度和光谱。本文介绍了一种计算模型,该模型整合了动力学电子物理学和原子过程,利用非平衡电子的玻尔兹曼方程和原子态布居的碰撞辐射模型。该模型用于研究非平衡电子对碰撞电离率的影响及其对布居分布的作用,正如在一个广为人知的实验中所观察到的那样[杨等人,《自然》(伦敦)466, 56 (2010)0028 - 083610.1038/nature09177]。研究表明,在X射线自由电子激光与物质相互作用期间存在显著的非平衡电子,这对气体等离子体中的碰撞电离率产生了深远影响,因此在应用于此类系统的碰撞辐射模型时需要仔细考虑。