Geophysical Prospecting and Surveying Team of Shandong Bureau of Coal Geological, Jinan, 250102, China.
College of Earth Science and Engineering, Shandong University of Science and Technology, Qingdao, 266590, China.
Environ Geochem Health. 2024 Sep 24;46(11):443. doi: 10.1007/s10653-024-02227-5.
To identify the sources of heavy metals in local soils and their risks to human health. This study quantified the concentrations of eight heavy metals in 504 soil samples collected in Tengzhou, China. The ecological risks of a single heavy metal (EI), a comprehensive ecological risk index (RI), and a health risk assessment model were used to evaluate the level of contamination in the city. The results of the research study indicate that there are different levels of heavy metal pollution in rural and urban agricultural areas in Tengzhou. Moreover, the spatial variability of mercury (Hg) is considerable, reaching 0.96, indicating a significant impact of anthropogenic activities. For the ecological risk, the heavy metal element with the highest EI value was mercury with a mean value of 67.22 and a peak value of 776.00. The heavy metal with the lowest mean EI value was Zn with only 1.03. Meanwhile, the average RI is only 128.59, but some areas have an RI as high as 842.2. The sources of heavy metals were identified using principal component analysis, correlation analysis, and an absolute principal component score multiple linear regression model (APCS-MLR). The non-carcinogenic risk for children, the carcinogenic risk for children, and the carcinogenic risk for adults were 1.23, 2.42×10 and 1.00×10, respectively, and these values exceeded their respective recommended values, and As and Cr had some carcinogenic hazards. Heavy metals in the soil come from natural, industrial, traffic and agricultural sources and represent 39.59%, 29.48%, 25.17% and 5.77%, respectively. The main source of heavy metals in local agricultural soils is the geological background, and the government needs to strengthen the monitoring of As and Cr in drinking water resources, as well as reduce traffic pollution and factory waste emissions to reduce Hg in soils.
为了识别当地土壤中重金属的来源及其对人类健康的风险。本研究在中国滕州采集了 504 个土壤样本,定量测定了其中 8 种重金属的浓度。采用单种重金属生态指数(EI)、综合生态风险指数(RI)和健康风险评估模型对城市污染程度进行评价。研究结果表明,滕州农村和城市农业区存在不同程度的重金属污染。此外,汞(Hg)的空间变异性较大,达到 0.96,表明人为活动的影响显著。在生态风险方面,EI 值最高的重金属元素是汞,平均值为 67.22,峰值为 776.00。EI 值最低的重金属元素是锌,平均值仅为 1.03。同时,平均 RI 仅为 128.59,但部分地区 RI 高达 842.2。利用主成分分析、相关分析和绝对主成分得分多元线性回归模型(APCS-MLR)确定重金属来源。儿童的非致癌风险、儿童的致癌风险和成人的致癌风险分别为 1.23、2.42×10 和 1.00×10,均超过各自的推荐值,砷(As)和铬(Cr)具有一定的致癌危害。土壤中的重金属来自自然、工业、交通和农业源,分别占 39.59%、29.48%、25.17%和 5.77%。当地农业土壤中重金属的主要来源是地质背景,政府需要加强对饮用水资源中 As 和 Cr 的监测,减少交通污染和工厂废物排放,以降低土壤中的 Hg。