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青藏高原沱沱河流域土壤中砷和其他元素的生态、环境风险及来源。

Ecological, environmental risks and sources of arsenic and other elements in soils of Tuotuo River region, Qinghai-Tibet Plateau.

机构信息

Key Laboratory of Natural Resource Coupling Process and Effects, Beijing, 100055, China.

Research Center of Applied Geology of China Geological Survey, Chengdu, 610039, China.

出版信息

Environ Geochem Health. 2024 Oct 1;46(11):460. doi: 10.1007/s10653-024-02161-6.

Abstract

Against the backdrop of global warming, the pollutants that were once "temporarily stored" in the permafrost are gradually being released, posing significant impacts on the environment. This has become an internationally focused hot topic. In this study, the contents of 11 elements such as As, Ti, Cd, Cr, Co, Mn, Cu, Pb, Ni, Zn and V in soil samples from 128 sampling points in the freeze-thaw area of the Tuotuo River in the source region of the Yangtze River on the Qinghai-Tibet Plateau were determined to evaluate the possible sources, contamination status and ecological, environmental and health risks of these elements. The mean values of As, Cd, Pb and Zn were higher than the corresponding Tibet soil background values. Among fourteen PTEs, As, Cd and Pb had the highest average values of enrichment factor and pollution index, indicating that freeze-thaw area soils showed moderate enrichment and pollution with As, Cd and Pb. Mean ecological risk factor (ER) of Cd was 109 and other PTEs mean ER values < 40, whereas ecological risk index (RI) values of all PTEs ranged from 59.5 to 880 and mean RI values was 152, indicating moderate ecological risk in study area. Explanatory power q value of total S (TS) content was 0.217 by GeogDetector, indicating TS was the most significant contributing factor to RI. Correlation analysis and PCA analysis showed that Cr, Cu, Ni, Co, Mn, Ti, V were mainly originated from natural sources, Cd, Pb and Zn from traffic activity, As from long-distance migration-freeze-thaw.

摘要

在全球变暖的背景下,曾经“暂时储存”在永久冻土中的污染物正在逐渐释放,对环境造成了重大影响。这已成为国际关注的热点话题。本研究对青藏高原长江源沱沱河冻融区 128 个采样点的土壤样品中 As、Ti、Cd、Cr、Co、Mn、Cu、Pb、Ni、Zn 和 V 等 11 种元素的含量进行了测定,以评价这些元素的可能来源、污染状况以及生态、环境和健康风险。As、Cd、Pb 和 Zn 的平均值高于相应的西藏土壤背景值。在 14 种 PTEs 中,As、Cd 和 Pb 的富集因子和污染指数平均值最高,表明冻融区土壤对 As、Cd 和 Pb 具有中等程度的富集和污染。Cd 的平均生态风险因子(ER)为 109,其他 PTEs 的平均 ER 值<40,而所有 PTEs 的生态风险指数(RI)值范围为 59.5 至 880,平均值为 152,表明研究区存在中度生态风险。总硫(TS)含量的 GeogDetector 解释力 q 值为 0.217,表明 TS 是 RI 的最主要贡献因素。相关分析和 PCA 分析表明,Cr、Cu、Ni、Co、Mn、Ti、V 主要来源于自然源,Cd、Pb 和 Zn 来源于交通活动,As 来源于长距离迁移-冻融。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/946d/11457720/a1ef0c60b1de/10653_2024_2161_Fig1_HTML.jpg

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