Cho Sangyeon, Martino Nicola, Yun Seok-Hyun
Wellman Center for Photomedicine, Massachusetts General Hospital, Cambridge, MA, USA.
Harvard Medical School, Boston, MA, USA.
Nat Nanotechnol. 2025 Mar;20(3):404-410. doi: 10.1038/s41565-024-01843-7. Epub 2025 Jan 2.
The ultimate limit for laser miniaturization would be achieving lasing action in the lowest-order cavity mode within a device volume of ≤(λ/2n), where λ is the free-space wavelength and n is the refractive index. Here we highlight the equivalence of localized surface plasmons and surface plasmon polaritons within resonant systems, introducing nanolasers that oscillate in the lowest-order localized surface plasmon or, equivalently, half-cycle surface plasmon polariton. These diffraction-limited single-mode emitters, ranging in size from 170 to 280 nm, harness strong coupling between gold and InGaAsP in the near-infrared (λ = 1,000-1,460 nm), away from the surface plasmon frequency. This configuration supports only the lowest-order dipolar mode within the semiconductor's broad gain bandwidth. A quasi-continuous-level semiconductor laser model explains the lasing dynamics under optical pumping. In addition, we fabricate isolated gold-coated semiconductor discs and demonstrate higher-order lasing within live biological cells. These plasmonic nanolasers hold promise for multi-colour imaging and optical barcoding in cellular applications.
激光微型化的最终极限将是在体积≤(λ/2n)的器件中以最低阶腔模实现激光作用,其中λ是自由空间波长,n是折射率。在此,我们强调共振系统中局域表面等离子体激元和表面等离子体激元极化激元的等效性,介绍了在最低阶局域表面等离子体激元或等效的半周期表面等离子体激元极化激元中振荡的纳米激光器。这些尺寸在170至280纳米之间的衍射极限单模发射器,利用了金与近红外(λ = 1000 - 1460纳米)的InGaAsP之间的强耦合,远离表面等离子体激元频率。这种配置在半导体的宽增益带宽内仅支持最低阶偶极模。一个准连续能级半导体激光模型解释了光泵浦下的激光动力学。此外,我们制造了孤立的镀金半导体圆盘,并在活体细胞内展示了高阶激光作用。这些等离子体纳米激光器在细胞应用中的多色成像和光学条形码方面具有潜力。