Fu Jianan, Li Xin, Li Zhen, Sun Fei, Wen Wenxin, Zhao Jinlai, Ruan Wenqing, Ren Shuai, Zhang Zhenxuan, Liang Xiong, Ma Jiang
Shenzhen Key Laboratory of High Performance Nontraditional Manufacturing, College of Mechatronics and Control Engineering, Shenzhen University, Shenzhen 518060, China.
College of Materials Science and Engineering, Shenzhen Key Laboratory of Polymer Science and Technology, Guangdong Research Center for Interfacial Engineering of Functional Materials, Shenzhen 518060, China.
Fundam Res. 2022 Oct 8;5(1):307-314. doi: 10.1016/j.fmre.2022.09.017. eCollection 2025 Jan.
Broadband light absorption is important for applications such as infrared detectors, solar energy collectors, and photothermal conversion. We propose a facile and common strategy to fabricate light absorbers with strong ultra-wideband absorption. Due to their excellent thermoplastic forming ability, metallic glasses could be patterned into finely arranged nanowire arrays, which show extremely low reflectivity (∼0.6%) in the visible and near-infrared regimes, and a low reflectivity (∼15%) in the mid-infrared regime as caused by multiscale nano spacing, multiple reflections, and plasmonic behavior. The strong absorption at surfaces with nanowires provides excellent photothermal conversion properties. The photothermal properties show that a surface with nanowires can be rapidly heated up to ∼160 °C at a rate of 28.75 °C/s, which is 30 times higher than smooth surfaces. Meanwhile, a surface with nanowires shows a high photothermal conversion efficiency ( = 56.36%). The fabricated metallic glass absorbers exhibit adaptability as they can be easily formed into various complex shapes and meet the requirements under harsh conditions. The outcomes of our research open the door to manufacturing high-performance absorbers for applications in photothermal electric power generation, desalination, and photodetectors.
宽带光吸收对于红外探测器、太阳能收集器和光热转换等应用至关重要。我们提出了一种简便且通用的策略来制造具有强超宽带吸收的光吸收体。由于其出色的热塑性成型能力,金属玻璃可以被加工成排列精细的纳米线阵列,这些阵列在可见光和近红外波段显示出极低的反射率(约0.6%),而在中红外波段由于多尺度纳米间距、多次反射和等离子体行为导致反射率较低(约15%)。具有纳米线的表面的强吸收提供了优异的光热转换性能。光热性能表明,具有纳米线的表面可以以28.75℃/s的速率迅速加热到约160℃,这比光滑表面高30倍。同时,具有纳米线的表面显示出高光热转换效率(=56.36%)。所制造的金属玻璃吸收体具有适应性,因为它们可以很容易地加工成各种复杂形状,并满足苛刻条件下的要求。我们的研究成果为制造用于光热发电、海水淡化和光电探测器应用的高性能吸收体打开了大门。