Gajda Roman, Chodkiewicz Michał, Zhang Dongzhou, Nguyen Phuong, Prakapenka Vitali, Wozniak Krzysztof
Biological and Chemical Research Centre, Department of Chemistry, University of Warsaw, Żwirki i Wigury 101, Warszawa 02-089, Poland.
GeoSoilEnviroCARS, University of Chicago, 9700 S. Cass Avenue, Argonne, IL 60439, USA.
IUCrJ. 2025 May 1;12(Pt 3):288-294. doi: 10.1107/S2052252525002581.
In the refinement of the crystal structures of ice, the best results obtained so far have been with neutron diffraction because the most troublemaking aspects are the hydrogen atoms. In nine out of twenty ice structures, the hydrogen atoms are disordered, which makes proper refinement more difficult. In our previous paper describing the structure of ice VI we proved that, using Hirshfeld atom refinement (HAR) based on synchrotron X-ray data, it is possible to obtain results comparable with those from neutron experiments. In this work, we investigate another structure of high-pressure disordered ice, cubo-ice (ice VII). Single crystals of cubo-ice were grown under pressure in diamond anvil cells. X-ray diffraction measurements were conducted at a synchrotron source facility (APS, University of Chicago, USA) as well as on our regular in-house laboratory diffractometer with Ag radiation. The data collected were further refined with HAR. Comparison of the structural parameters obtained with those derived from neutron diffraction showed very good agreement in terms of bond lengths and fairly good agreement in terms of hydrogen atom ADPs. We were also able to perform unconstrained refinements with various split-atom models.
在冰晶体结构的精修中,目前为止获得的最佳结果是通过中子衍射得到的,因为最棘手的方面是氢原子。在二十种冰结构中的九种里,氢原子是无序的,这使得进行适当的精修更加困难。在我们之前描述冰VI结构的论文中,我们证明了,使用基于同步加速器X射线数据的 Hirshfeld 原子精修(HAR),有可能获得与中子实验结果相当的结果。在这项工作中,我们研究了另一种高压无序冰的结构——立方冰(冰VII)。立方冰的单晶在金刚石对顶砧池中加压生长。在美国芝加哥大学的同步加速器源设施(APS)以及我们常规的内部实验室衍射仪上,使用银辐射进行了X射线衍射测量。收集到的数据用HAR进一步精修。将获得的结构参数与从中子衍射得出的参数进行比较,结果表明在键长方面非常吻合,在氢原子各向异性位移参数方面相当吻合。我们还能够使用各种分裂原子模型进行无约束精修。