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基于丙酮的新型锂负载液体闪烁体。

Lithium-loaded acetone-based novel liquid scintillator.

作者信息

Kang Tae Yeong, Choi Ji Young, Joo Kyung Kwang, Kim Eun Min, Kim Sang Yong

机构信息

Center for Precision Neutrino Research, Department of Physics, Chonnam National University, Yongbongro 77, Pukgu, 61186, Gwangju, Republic of Korea.

出版信息

Sci Rep. 2025 Jul 25;15(1):27042. doi: 10.1038/s41598-025-12985-6.

Abstract

Liquid scintillators are widely used in diverse fields because they can be easily synthesized and offer high light yield. Therefore, developing a stable liquid scintillator is crucial. In this study, we synthesized a novel liquid scintillator using acetone as a base solvent and measured its physical and optical properties. The optimal mixing ratio of acetone, water, and fluors constituting the liquid scintillator was investigated. Although acetone is a polar solution, we noticed that it also exhibits non-polar properties and used it to synthesize lithium-loaded liquid scintillator. This is a completely new method to load lithium by taking advantage of the amphiphilicity of acetone. In addition, neutron and gamma discrimination was attempted by loading enriched [Formula: see text]Li, which has a large neutron capture cross section. Unlike that in previous studies, no strong hydrochloric acid, surfactants, or any other solubilizing additions are required when loading [Formula: see text]Li. A 100 ml glass cell was filled with our liquid scintillator and irradiated with [Formula: see text]Cf radioactive source. For neutron and gamma discrimination, conventional pulse shape discrimination method was used. To the best of our knowledge, no previous study has attempted a liquid scintillator using acetone, and this type of product is not available at all in the current market up to now. Nonetheless, there is still room to improve and potential for a new type of development in this field. We believe that these results have potential applications in next-generation particle, nuclear, and medical physics experiments.

摘要

液体闪烁体因其易于合成且光产额高而被广泛应用于各种领域。因此,开发一种稳定的液体闪烁体至关重要。在本研究中,我们以丙酮为基础溶剂合成了一种新型液体闪烁体,并测量了其物理和光学性质。研究了构成液体闪烁体的丙酮、水和荧光体的最佳混合比例。尽管丙酮是一种极性溶液,但我们注意到它也表现出非极性性质,并利用它来合成载锂液体闪烁体。这是一种利用丙酮的两亲性来载锂的全新方法。此外,通过装载具有大中子俘获截面的富集[化学式:见原文]锂来尝试进行中子和伽马射线鉴别。与以往研究不同的是,装载[化学式:见原文]锂时不需要强盐酸、表面活性剂或任何其他增溶添加剂。一个100毫升的玻璃容器装满我们的液体闪烁体,并用[化学式:见原文]Cf放射源进行辐照。对于中子和伽马射线鉴别,使用了传统的脉冲形状鉴别方法。据我们所知,以前没有研究尝试过使用丙酮的液体闪烁体,而且到目前为止这种产品在当前市场上根本不存在。尽管如此,该领域仍有改进空间和新型开发的潜力。我们相信这些结果在下一代粒子、核和医学物理实验中具有潜在应用。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/00ea/12297494/51609d398a47/41598_2025_12985_Fig1_HTML.jpg

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