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Selective triggering in-plane and out-of-plane dipolar modes of hexagonal Au nanoplate with the polarization of excitation beam.

作者信息

Zhang Hanmou, Wang Qifa, Hou Liping, Xiao Fajun, Zhao Jianlin

机构信息

Key Laboratory of Light Field Manipulation and Information Acquisition, Ministry of Industry and Information Technology, and Shaanxi Key Laboratory of Optical Information Technology, School of Physical Science and Technology, Northwestern Polytechnical University, Xi'an 710129, People's Republic of China.

出版信息

J Phys Condens Matter. 2022 Nov 1;34(50). doi: 10.1088/1361-648X/ac9d18.

Abstract

The dipolar responses of a single hexagonal Au nanoplate are investigated under the illuminations of linearly polarized beam and tightly focused radially polarized beam (RPB). It is found from the scattering spectra that the in-plane and out-of-plane electric dipole modes can be selectively triggered with a linearly polarized beam and tightly focused RPB, respectively. The features of these two dipolar modes are further confirmed in terms of electrical field and charge maps by the finite-difference time-domain simulation. Additionally, using the multipole expansion method, the existence of the out-of-plane dipole mode is further verified by the fact that the-component of electric dipole response has a dominant contribution to the scattered power. Moreover, by combining the back focal plane imaging technique with the simulation, the appearance of in-plane and out-of-plane dipoles in the scattering pattern are clearly discerned. Our results provide an efficient method for selectively exciting the in-plane and out-of-plane dipolar modes of the nanoplate. We envision that the ease of tuning the dipolar momentum may facilitate the enhancement of the interaction between the plasmon and emitters at single-particle level.

摘要

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