Tsubery H, Ofek I, Cohen S, Fridkin M
Department of Organic Chemistry, The Weizmann Institute of Science, Rehovot, 76100, Israel.
Biochemistry. 2000 Oct 3;39(39):11837-44. doi: 10.1021/bi000386q.
The Gram-negative bacterial endotoxin lipopolysaccharide (LPS) is a major inducer of sepsis. The natural cyclic peptide polymyxin B (PMB) is a potent antimicrobial agent, albeit highly toxic, by virtue of its capacity to neutralize the devastating effects of LPS. However, the exact mode of association between PMB and LPS is not clear. In this study, we have synthesized polymyxin B nonapeptide, the LPS-binding cyclic domain of PMB, and its enantiomeric analogue and studied several parameters related to their interaction with LPS and their capacity to sensitize Gram-negative bacteria toward hydrophobic antibiotics. The results suggest that whereas the binding of the two enantiomeric peptides to E. coli and to E. coli LPS is rather similar, functional association with the bacterial cell is stereospecific. Thus, the L-enantiomer is capable of synergism with the hydrophobic antimicrobial drugs novobiocin and erythromycin, whereas the D-enantiomer is devoid of such activity. The potential of understanding and consequently utilizing the PMB-LPS association for novel, nontoxic PMB-derived drugs is discussed.
革兰氏阴性菌内毒素脂多糖(LPS)是脓毒症的主要诱导物。天然环肽多粘菌素B(PMB)是一种强效抗菌剂,尽管毒性很强,但因其能够中和LPS的破坏性作用。然而,PMB与LPS之间的确切结合方式尚不清楚。在本研究中,我们合成了多粘菌素B九肽(PMB的LPS结合环域)及其对映体类似物,并研究了与它们与LPS相互作用以及使革兰氏阴性菌对疏水性抗生素敏感的能力相关的几个参数。结果表明,虽然两种对映体肽与大肠杆菌和大肠杆菌LPS的结合相当相似,但与细菌细胞的功能关联具有立体特异性。因此,L-对映体能够与疏水性抗菌药物新生霉素和红霉素产生协同作用,而D-对映体则没有这种活性。本文讨论了理解并因此利用PMB-LPS关联开发新型无毒PMB衍生药物的潜力。