Lein M, Gross EK, Engel V
Institut fur Physikalische Chemie, Am Hubland, 97074 Wurzburg, Germany and Institut fur Theoretische Physik, Am Hubland, 97074 Wurzburg, Germany.
Phys Rev Lett. 2000 Nov 27;85(22):4707-10. doi: 10.1103/PhysRevLett.85.4707.
We present quantum mechanical calculations of the electron and ion momentum distributions following double ionization of a one-dimensional helium atom by ultrashort laser pulses (780 nm) at various intensities. The two-electron momentum distributions exhibit a clear transition from nonsequential to sequential double ionization. We provide strong evidence that rescattering is responsible for nonsequential ionization by calculating the momentum spectrum of the He2+ recoil ions-which we find in excellent agreement with recent experiments-and by analyzing the electronic center-of-mass motion via Wigner transforms.
我们展示了在不同强度的超短激光脉冲(780纳米)作用下,一维氦原子双电离后电子和离子动量分布的量子力学计算结果。双电子动量分布呈现出从非顺序双电离到顺序双电离的清晰转变。通过计算He2+反冲离子的动量谱(我们发现其与最近的实验结果高度吻合)以及通过维格纳变换分析电子质心运动,我们提供了有力证据表明再散射是导致非顺序电离的原因。