Lipowski A, Johnston D
Department of Mathematics, Heriot-Watt University, EH14 4AS Edinburgh, United Kingdom and Department of Physics, A. Mickiewicz University, 61-614 Poznan, Poland.
Phys Rev E Stat Phys Plasmas Fluids Relat Interdiscip Topics. 2000 Jun;61(6 Pt A):6375-82. doi: 10.1103/physreve.61.6375.
Using Monte Carlo simulations we study cooling-rate effects in a three-dimensional Ising model with four-spin interactions. During coarsening, this model develops growing energy barriers, which at low temperature lead to very slow dynamics. We show that the characteristic zero-temperature length increases very slowly with the inverse cooling rate, similarly to the behavior of ordinary glasses. For computationally accessible cooling rates the model undergoes an ideal glassy transition, i.e., the glassy transition for a very small cooling rate coincides with a thermodynamic singularity. We also study the cooling of this model with a certain fraction of spins fixed. Due to such heterogeneous crystallization seeds, the final state strongly depends on the cooling rate. Only for a sufficiently fast cooling rate does the system end up in a glassy state, while slow cooling inevitably leads to a crystal phase.
我们使用蒙特卡罗模拟研究了具有四自旋相互作用的三维伊辛模型中的冷却速率效应。在粗化过程中,该模型会形成不断增长的能垒,在低温下这会导致动力学非常缓慢。我们表明,特征零温长度随冷却速率的倒数增加得非常缓慢,这与普通玻璃的行为类似。对于计算上可及的冷却速率,该模型经历理想的玻璃态转变,即非常小的冷却速率下的玻璃态转变与热力学奇点重合。我们还研究了固定一定比例自旋时该模型的冷却情况。由于这种异质结晶种子,最终状态强烈依赖于冷却速率。只有冷却速率足够快时,系统最终才会处于玻璃态,而缓慢冷却不可避免地会导致晶相。