Chuang Y D, Gromko A D, Dessau D S, Kimura T, Tokura Y
Department of Physics, University of Colorado, Boulder, CO 80309-0390, USA.
Science. 2001 May 25;292(5521):1509-13. doi: 10.1126/science.1059255. Epub 2001 Apr 26.
We used high-resolution angle-resolved photoemission spectroscopy to reveal the Fermi surface and key transport parameters of the metallic state of the layered colossal magnetoresistive oxide La1.2Sr1.8Mn2O7. With these parameters, the calculated in-plane conductivity is nearly one order of magnitude larger than the measured direct current conductivity. This discrepancy can be accounted for by including the pseudogap, which removes at least 90% of the spectral weight at the Fermi energy. Key to the pseudogap and to many other properties are the parallel straight Fermi surface sections, which are highly susceptible to nesting instabilities. These nesting instabilities produce nanoscale fluctuating charge/orbital modulations, which cooperate with Jahn-Teller distortions and compete with the electron itinerancy favored by double exchange.
我们使用高分辨率角分辨光电子能谱来揭示层状巨磁电阻氧化物La1.2Sr1.8Mn2O7金属态的费米面和关键输运参数。利用这些参数,计算出的面内电导率比测量的直流电导率大近一个数量级。这种差异可以通过引入赝能隙来解释,赝能隙消除了费米能处至少90%的谱权重。赝能隙以及许多其他性质的关键在于平行的直费米面截面,这些截面极易受到嵌套不稳定性的影响。这些嵌套不稳定性产生纳米级的波动电荷/轨道调制,它们与 Jahn-Teller 畸变相互作用,并与双交换所青睐的电子巡游性相互竞争。