Soderberg T, Chen A, Poulter C D
Department of Chemistry, University of Utah, Salt Lake City, Utah 84112, USA.
Biochemistry. 2001 Dec 11;40(49):14847-54. doi: 10.1021/bi0111799.
Geranylgeranylglyceryl diphosphate synthase (GGGP synthase) catalyzes alkylation of (S)-glyceryl phosphate [(S)-GP] by geranylgeranyl diphosphate (GGPP) to produce (S)-geranylgeranylglyceryl phosphate [(S)-GGGP]. This reaction is the first committed step in the biosynthesis of ether-linked membrane lipids in Archaea. The gene encoding GGGP synthase from Methanobacterium thermoautotrophicum was cloned using probes designed from the N-terminal sequence determined from the purified enzyme. The open reading frame, which encoded a protein of 245 amino acids, was inserted into a pET expression vector and expressed in Escherichia coli. The recombinant GGGP synthase was purified to homogeneity. The enzyme is active as a homopentamer, as determined by size exclusion chromatography and equilibrium sedimentation experiments. GGGP synthase has optimal activity at 55 degrees C in pH 8.0 buffer containing 1 mM MgCl(2). V(max) = 4.0 +/- 0.1 micromol min(-1) mg(-1) (k(cat) = 0.34 +/- 0.03 s(-1) for pentameric GGGP synthase assuming all subunits are fully active), K(m)((S)-GP) = 13.5 +/- 1.0 microM, and K(m)(GGPP) = 506 +/- 47 nM. These steady-state catalytic constants were identical to those for enzyme isolated from cell extracts of M. thermoautotrophicum [Chen, A., Zhang, D., and Poulter, C. D. (1993) J. Biol. Chem. 268, 21701-21705]. Alignment of seven putative archaeal GGGP synthase sequences revealed a number of highly conserved residues consisting of five aspartate/glutamates, three serine/threonines, two prolines, and five glycines, including a conserved GGG motif.
香叶基香叶基甘油二磷酸合酶(GGGP合酶)催化香叶基香叶基二磷酸(GGPP)对(S)-甘油磷酸[(S)-GP]进行烷基化反应,生成(S)-香叶基香叶基甘油磷酸[(S)-GGGP]。该反应是古菌中醚键连接膜脂生物合成的第一个关键步骤。利用根据从纯化酶中确定的N端序列设计的探针,克隆了嗜热自养甲烷杆菌中编码GGGP合酶的基因。将编码245个氨基酸的开放阅读框插入pET表达载体,并在大肠杆菌中表达。重组GGGP合酶被纯化至同质。通过尺寸排阻色谱和平衡沉降实验确定,该酶作为同五聚体具有活性。GGGP合酶在含1 mM MgCl₂的pH 8.0缓冲液中,于55℃时具有最佳活性。V(max)=4.0±0.1 μmol min⁻¹ mg⁻¹(假设所有亚基均完全有活性,五聚体GGGP合酶的k(cat)=0.34±0.03 s⁻¹),K(m)[(S)-GP]=13.5±1.0 μM,K(m)(GGPP)=506±47 nM。这些稳态催化常数与从嗜热自养甲烷杆菌细胞提取物中分离得到的酶的常数相同[Chen, A., Zhang, D., and Poulter, C. D. (1993) J. Biol. Chem. 268, 21701 - 21705]。对七个假定的古菌GGGP合酶序列进行比对,发现了许多高度保守的残基,包括五个天冬氨酸/谷氨酸、三个丝氨酸/苏氨酸、两个脯氨酸和五个甘氨酸,其中包括一个保守的GGG基序。