Zhao J, Li N, Warren P V, Golbeck J H, Bryant D A
Department of Molecular and Cell Biology, Pennsylvania State University, University Park 16802.
Biochemistry. 1992 Jun 9;31(22):5093-9. doi: 10.1021/bi00137a001.
The terminal electron acceptors FA and FB exist as two [4Fe-4S] clusters located on the 8.9-kDa PsaC protein in photosystem I. We have used site-directed mutagenesis to produce a complementary pair of mutant PsaC proteins in which specific cysteine ligands to the [4Fe-4S] clusters were changed to aspartic acid residues. The mutant proteins, denoted C14D and C51D, were overproduced in Escherichia coli; the iron-sulfur clusters were inserted in vitro; and the reconstituted proteins were rebound to the P700-FX core of Synechococcus sp. PCC 6301 in the presence of the PsaD protein. In complexes reconstituted with C51D a rhombic ESR spectrum with g-values of 2.063, 1.934, and 1.879 in the reduced state identifies the intact [4Fe-4S] cluster as FB, while an intense axial spectrum with g-values of 2.020 and 1.997 in the oxidized state identifies the altered cluster in the aspartate site as a [3Fe-4S] cluster. The [3Fe-4S] cluster corresponding to FA can be reduced chemically with dithionite and photochemically by illumination at room temperature but is not reduced by illumination at 15 K. With reconstituted C14D a rhombic ESR spectrum with g-values of 2.043, 1.942, and 1.853 in the reduced state identified the unaltered [4Fe-4S] cluster as FA, while a complex spectrum with a gz-value of 2.194 and an asymmetric gx,y set of resonances between 2.092 and 1.999 indicates an altered cluster of unknown identity in the site containing the aspartate ligand. The ESR signals arising from the altered cluster corresponding to FB are not diminished by illumination at either room temperature or 15 K.(ABSTRACT TRUNCATED AT 250 WORDS)
末端电子受体FA和FB以两个[4Fe-4S]簇的形式存在,位于光系统I中8.9 kDa的PsaC蛋白上。我们利用定点诱变产生了一对互补的突变PsaC蛋白,其中与[4Fe-4S]簇特异性结合的半胱氨酸配体被替换为天冬氨酸残基。这两种突变蛋白分别命名为C14D和C51D,在大肠杆菌中过量表达;铁硫簇在体外插入;重组蛋白在PsaD蛋白存在的情况下与集胞藻PCC 6301的P700-FX核心重新结合。在用C51D重组的复合物中,还原态下g值为2.063、1.934和1.879的菱形电子顺磁共振(ESR)光谱表明完整的[4Fe-4S]簇为FB,而氧化态下g值为2.020和1.997的强烈轴向光谱表明天冬氨酸位点改变后的簇为[3Fe-4S]簇。对应于FA的[3Fe-4S]簇可以用连二亚硫酸盐进行化学还原,在室温下通过光照进行光化学还原,但在15 K光照下不能还原。在用重组C14D时,还原态下g值为2.043、1.942和1.853的菱形ESR光谱表明未改变的[4Fe-4S]簇为FA,而gz值为2.194且gx,y共振不对称集在2.092和1.999之间的复杂光谱表明在含有天冬氨酸配体的位点有一个身份未知的改变后的簇。对应于FB的改变后的簇产生的ESR信号在室温或15 K光照下均未减弱。(摘要截选至250字)