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波兰公共饮用水中的铀同位素及人体剂量评估

Uranium isotopes in public drinking water and dose assessment for man in Poland.

作者信息

Pietrzak-Flis Zofia, Kaminska Iwona, Chrzanowski Edward

机构信息

Central Laboratory for Radiological Protection, Konwaliowa 7, 03-194 Warsaw, Poland.

出版信息

Radiat Prot Dosimetry. 2005;113(1):34-9. doi: 10.1093/rpd/nch425. Epub 2004 Nov 23.

Abstract

238U, 234U and 235U were determined in tap water from municipal water pipes that drew their supply from surface water or ground water in various locations in Poland. Average activity concentrations of 238U, 234U and 235U in tap water from surface water were 9.6 +/- 7.1, 12.8 +/- 9.7 and 0.41 +/- 0.31 Bq m(-3), respectively, whereas from ground water they were 4.5 +/- 6.0, 5.7 +/- 6.9 and 0.19 +/- 0.27 Bq m(-3), respectively. Activity concentrations of 234U were higher than 238U. Ratios of 234U/238U ranged from 1.07 to 2.60, indicating the lack of equilibrium between these isotopes. The average 235U/238U ratio was 0.043 +/- 0.008, being close to 0.046 for natural uranium. Average annual intake with water and food was 7.6 +/- 5.1 Bq for 238U and 9.5 +/- 6.6 Bq for 234U. Annual committed effective doses calculated from these intakes for adults were 0.34 +/- 0.23 and 0.47 +/- 0.32 microSv, respectively; 235U contributed to the total dose from the uranium isotopes by about 2%.

摘要

对取自波兰各地地表水或地下水的市政供水管道中的自来水进行了238U、234U和235U的测定。取自地表水的自来水中238U、234U和235U的平均活度浓度分别为9.6±7.1、12.8±9.7和0.41±0.31 Bq m(-3),而取自地下水的分别为4.5±6.0、5.7±6.9和0.19±0.27 Bq m(-3)。234U的活度浓度高于238U。234U/238U的比值在1.07至2.60之间,表明这些同位素之间缺乏平衡。235U/238U的平均比值为0.043±0.008,接近天然铀的0.046。238U通过水和食物的年平均摄入量为7.6±5.1 Bq,234U为9.5±6.6 Bq。根据这些摄入量计算出的成人年待积有效剂量分别为0.34±0.23和0.47±0.32 μSv;235U对铀同位素总剂量的贡献约为2%。

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