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Spatiotemporal patterns of external noise-induced transitions in a bistable reaction-diffusion system: photoelectron emission microscopy experiments and modeling.

作者信息

Wehner Stefan, Hoffmann Patrick, Schmeisser Dieter, Brand Helmut R, Küppers Jürgen

机构信息

Experimentalphysik III, Universität Bayreuth, 95440 Bayreuth, Germany.

出版信息

Phys Rev Lett. 2005 Jul 15;95(3):038301. doi: 10.1103/PhysRevLett.95.038301. Epub 2005 Jul 11.

Abstract

The rate of CO oxidation on Ir(111) surfaces exhibits bistability at T=500 K in a range of the CO fraction Y in the CO+O reactant gas flux. Measured CO2 rates as a function of the noise strength imposed on Y are well reproduced by parameter-free modeling. We present photoelectron emission microscopy measurements and 2D calculations of the spatiotemporal patterns of CO- and O-rich domains. The role of combined multiplicative and additive noise on Y for CO and O domain wall motion and island nucleation-growth-coalescence processes is analyzed.

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