Ye Dan, Gao Dengshan, Yu Gang, Shen Xianglin, Gu Fan
Education Ministry Key Laboratory on Clean Coal Power Generation and Combustion Technology, Southeast University, Nanjing, China.
J Hazard Mater. 2005 Dec 9;127(1-3):149-55. doi: 10.1016/j.jhazmat.2005.06.040. Epub 2005 Aug 29.
A plasma reactor with catalysts was used to treat exhaust gas from a gasoline engine in order to decrease particulate matter (PM) emissions. The effect of non-thermal plasma (NTP) of the dielectric discharges on the removal of PM from the exhaust gas was investigated experimentally. The removal efficiency of PM was based on the concentration difference in PM for particle diameters ranging from 0.3 to 5.0 microm as measured by a particle counter. Several factors affecting PM conversion, including the density of plasma energy, reaction temperature, flow rate of exhaust gas, were investigated in the experiment. The results indicate that PM removal efficiency ranged approximately from 25 to 57% and increased with increasing energy input in the reactor, reaction temperature and residence time of the exhaust gas in the reactor. Enhanced removal of the PM was achieved by filling the discharge gap of the reactor with Cu-ZSM-5 catalyst pellets. In addition, the removal of unburned hydrocarbons was studied. Finally, available approaches for PM conversion were analyzed involving the interactions between discharge and catalytic reactions.
采用带有催化剂的等离子体反应器处理汽油发动机的废气,以降低颗粒物(PM)排放。实验研究了介质放电产生的非热等离子体(NTP)对废气中PM去除的影响。PM的去除效率基于颗粒计数器测量的直径范围为0.3至5.0微米的PM浓度差。实验研究了影响PM转化的几个因素,包括等离子体能量密度、反应温度、废气流量。结果表明,PM去除效率约为25%至57%,并随着反应器中能量输入、反应温度和废气在反应器中的停留时间的增加而提高。通过在反应器的放电间隙中填充Cu-ZSM-5催化剂颗粒,实现了PM的增强去除。此外,还研究了未燃烧碳氢化合物的去除。最后,分析了涉及放电与催化反应相互作用的PM转化可用方法。