Gorecka J, Gorecki J
Institute of Physics, Polish Academy of Sciences, Al. Lotnikow 36/42, 02-668, Warsaw, Poland.
Phys Chem Chem Phys. 2005 Aug 7;7(15):2915-20. doi: 10.1039/b504621a. Epub 2005 Jul 6.
The oxidation of carbon monoxide on a Pt(110) surface is considered as a medium for chemical information processing in which bits of information are represented by traveling pulses of high oxygen coverage. Using numerical simulations for a model of CO oxidation we demonstrate that in such system one dimensional chemical signal diode can be realized by setting a proper profile of temperature. We also show that a pulse splitting can occur on a temperature inhomogeneity. The phenomenon of pulse splitting can be used to construct one dimensional generator of a train of pulses with adjustable frequency.
一氧化碳在Pt(110)表面的氧化被视为一种化学信息处理介质,其中信息位由高氧覆盖率的传播脉冲表示。通过对一氧化碳氧化模型进行数值模拟,我们证明在这样的系统中,通过设置合适的温度分布可以实现一维化学信号二极管。我们还表明,在温度不均匀性上会发生脉冲分裂。脉冲分裂现象可用于构建频率可调的脉冲序列一维发生器。