Joshi Bhalchandra V, Jacobson Kenneth A
Molecular Recognition Section, Laboratory of Bioorganic Chemistry, National Institute of Diabetes and Digestive and Kidney Diseases, National Institutes of Health, Bethesda, Maryland 20892, USA.
Curr Top Med Chem. 2005;5(13):1275-95. doi: 10.2174/156802605774463079.
Selective agonists and antagonists for A3 adenosine receptors (ARs) are being explored for the treatment of a variety of disorders, including brain and heart ischemic conditions, cancer, and rheumatoid arthritis. This review covers both the structure activity relationships of nucleoside agonist ligands and selected antagonists acting at this receptor and the routes of synthesis. Highly selective agonists have been designed, using both empirical approaches and a semi-rational approach based on molecular modeling. The prototypical A3 agonists IB-MECA 10 and the more receptor-subtype-selective Cl-IB-MECA 11, both of which have affinity in binding to the receptor of approximately 1 nM, have been used widely as pharmacological probes in the elucidation of the physiological role of this receptor. In addition to the exploration of the effects of structural modification of the adenine and ribose moieties on A3AR affinity, the effects of these structural changes on the intrinsic efficacy have also been studied in a systematic fashion. Key structural features determining A3AR interaction include the N6-benzyl group, 2-position substitution such as halo, substitution of ribose (e.g., the (N)-methanocarba ring system, various 2'- and 3'-substitutions and 4'-thio substitution of oxygen). Conformational studies of the ribose moiety and its equivalents indicate that the ring oxygen is not required and the North (N) ring conformation is preferred in binding to the A3AR. Using these observations, a series of ring constrained (N)-methanocarba 5'-uronamide derivatives was recently reported to be highly selective A3AR agonists, the most notable amongst them was MRS3558 113 having a Ki value in binding to the human A3 receptor of 0.3 nM.
A3腺苷受体(AR)的选择性激动剂和拮抗剂正在被研究用于治疗多种疾病,包括脑和心脏缺血性疾病、癌症和类风湿性关节炎。本综述涵盖了核苷激动剂配体和作用于该受体的选定拮抗剂的构效关系以及合成路线。已经采用经验方法和基于分子建模的半理性方法设计出了高选择性激动剂。原型A3激动剂IB-MECA 10和受体亚型选择性更高的Cl-IB-MECA 11,二者与该受体结合的亲和力均约为1 nM,已被广泛用作药理学探针以阐明该受体的生理作用。除了探索腺嘌呤和核糖部分的结构修饰对A3AR亲和力的影响外,还系统地研究了这些结构变化对内在活性的影响。决定A3AR相互作用的关键结构特征包括N6-苄基、2-位取代如卤代、核糖取代(例如(N)-甲碳环系统、各种2'-和3'-取代以及4'-硫代取代氧)。核糖部分及其等效物的构象研究表明,环氧化合物并非必需,并且在与A3AR结合时,北(N)环构象更受青睐。基于这些观察结果,最近报道了一系列环约束(N)-甲碳环5'-脲酰胺衍生物是高选择性A3AR激动剂,其中最显著的是MRS3558 113,其与人A3受体结合的Ki值为0.3 nM。