Hirasawa Masakazu, Nakayama Masato, Kim Sung-Kun, Hase Toshiharu, Knaff David B
Department of Chemistry and Biochemistry and Center for Biotechnology and Genomics, Texas Tech University, Lubbock, TX 79409-1061, USA.
Photosynth Res. 2005 Dec;86(3):325-36. doi: 10.1007/s11120-005-6966-y. Epub 2005 Nov 12.
The ferredoxin-dependent sulfite reductase from maize was treated, in separate experiments, with three different covalent modifiers of specific amino acid side chains. Treatment with the tryptophan-modifying reagent, N-bromosuccinimide (NBS), resulted in a loss of enzymatic activity with both the physiological donor for the enzyme, reduced ferredoxin, and with reduced methyl viologen, a non-physiological electron donor. Formation of the 1:1 ferredoxin/sulfite reductase complex prior to treating the enzyme with NBS completely protected the enzyme against the loss of both activities. Neither the secondary structure, nor the oxidation-reduction midpoint potential (Em) values of the siroheme and [4Fe-4S] cluster prosthetic groups of sulfite reductase, nor the binding affinity of the enzyme for ferredoxin were affected by NBS treatment. Treatment of sulfite reductase with the lysine-modifying reagent, N-acetylsuccinimide, inhibited the ferredoxin-linked activity of the enzyme without inhibiting the methyl viologen-linked activity. Complex formation with ferredoxin protects the enzyme against the inhibition of ferredoxin-linked activity produced by treatment with N-acetylsuccinimide. Treatment of sulfite reductase with N-acetylsuccinimide also decreased the binding affinity of the enzyme for ferredoxin. Treatment of sulfite reductase with the arginine-modifying reagent, phenylglyoxal, inhibited both the ferredoxin-linked and methyl viologen-linked activities of the enzyme but had a significantly greater effect on the ferredoxin-dependent activity than on the reduced methyl viologen-linked activity. The effects of these three inhibitory treatments are consistent with a possible role for a tryptophan residue the catalytic mechanism of sulfite reductase and for lysine and arginine residues at the ferredoxin-binding site of the enzyme.
在不同的实验中,用三种针对特定氨基酸侧链的不同共价修饰剂处理了玉米中的铁氧化还原蛋白依赖性亚硫酸盐还原酶。用色氨酸修饰剂N-溴代琥珀酰亚胺(NBS)处理后,该酶对于其生理供体还原型铁氧化还原蛋白以及非生理电子供体还原型甲基紫精的酶活性均丧失。在用NBS处理该酶之前形成1:1的铁氧化还原蛋白/亚硫酸盐还原酶复合物,可完全保护该酶的这两种活性不丧失。NBS处理既不影响亚硫酸盐还原酶的二级结构,也不影响其西罗血红素和[4Fe-4S]簇辅基的氧化还原中点电位(Em)值,也不影响该酶对铁氧化还原蛋白的结合亲和力。用赖氨酸修饰剂N-乙酰琥珀酰亚胺处理亚硫酸盐还原酶,可抑制该酶与铁氧化还原蛋白相关的活性,但不抑制与甲基紫精相关的活性。与铁氧化还原蛋白形成复合物可保护该酶免受N-乙酰琥珀酰亚胺处理所产生的对与铁氧化还原蛋白相关活性的抑制。用N-乙酰琥珀酰亚胺处理亚硫酸盐还原酶还降低了该酶对铁氧化还原蛋白的结合亲和力。用精氨酸修饰剂苯乙二醛处理亚硫酸盐还原酶,可抑制该酶与铁氧化还原蛋白相关的活性和与甲基紫精相关的活性,但对与铁氧化还原蛋白相关的活性的影响比对还原型甲基紫精相关活性的影响要大得多。这三种抑制处理的效果与色氨酸残基在亚硫酸盐还原酶催化机制中以及赖氨酸和精氨酸残基在该酶铁氧化还原蛋白结合位点中可能发挥的作用一致。