Chen R, Lo D, Lawless J L
School of Physics and Astronomy, Raymond and Beverly Sackler Faculty of Exact Sciences, Tel Aviv University, Tel-Aviv 69978, Israel.
Radiat Prot Dosimetry. 2006;119(1-4):33-6. doi: 10.1093/rpd/nci599. Epub 2006 Apr 27.
The thermoluminescence (TL) intensity in different materials is usually a monotonic increasing function of the dose, which quite often reaches a saturation value. In several materials, however, non-monotonic dose dependence has been observed. The TL intensity reached a maximum at a certain dose and decreased at higher ones. Some authors refer to this effect as 'radiation damage'. In the present work, we show that the non-monotonic dependence can easily be demonstrated to result from competition between transitions model with two trapping states and two kinds of recombination centres. Two kinds of competition are considered. One in which competition during excitation dominates, the filling of the active luminescence centre is non-monotonic, and the resulting TL is non-monotonic. In the other, the filling of traps and centres is monotonically increasing, but the competition during heating causes TL intensity to reach a maximum and decline at higher doses.
不同材料中的热释光(TL)强度通常是剂量的单调递增函数,且常常会达到一个饱和值。然而,在几种材料中,已观察到非单调的剂量依赖性。TL强度在某一剂量处达到最大值,而在更高剂量时则下降。一些作者将这种效应称为“辐射损伤”。在本工作中,我们表明非单调依赖性很容易被证明是由具有两个俘获态和两种复合中心的跃迁模型之间的竞争导致的。考虑了两种竞争。一种是激发过程中的竞争占主导,活性发光中心的填充是非单调的,从而产生的TL也是非单调的。另一种情况是,陷阱和中心的填充是单调增加的,但加热过程中的竞争导致TL强度在更高剂量时达到最大值并下降。