Miyake Yusuke, Takahashi Masahiko, Watanabe Noboru, Khajuria Yugal, Udagawa Yasuo, Sakai Yasuhiro, Mukoyama Takeshi
Institute of Multidisciplinary Research for Advanced Materials, Tohoku University, Sendai 980-8577, Japan.
Phys Chem Chem Phys. 2006 Jul 7;8(25):3022-8. doi: 10.1039/b603117j. Epub 2006 May 3.
Momentum profiles have been measured for the two outermost atomic orbitals of noble gases, Ar, Kr and Xe, at incident electron energy of about 2 keV using a newly developed multichannel (e,2e) spectrometer. The experimental results exhibit significantly improved statistics compared with those achieved in previous studies while covering a wide range of momenta up to 3.6 a.u. The results are compared with theoretical calculations using four (e,2e) scattering models, the plane-wave impulse and Born approximations (PWIA and PWBA), and the distorted-wave impulse and Born approximations (DWIA and DWBA). The DWIA and DWBA scattering models have been found to satisfactorily reproduce the experimental momentum profiles in terms of both shape and intensity over the entire momentum range covered, indicating the importance of distorted wave effects for quantitatively describing (e,2e) reaction.
利用新开发的多通道(e,2e)光谱仪,在约2 keV的入射电子能量下,测量了稀有气体氩、氪和氙的两个最外层原子轨道的动量分布。与之前的研究相比,实验结果的统计数据有了显著改善,同时覆盖了高达3.6 a.u.的广泛动量范围。将结果与使用四种(e,2e)散射模型的理论计算进行了比较,即平面波冲量近似和玻恩近似(PWIA和PWBA),以及扭曲波冲量近似和玻恩近似(DWIA和DWBA)。已发现DWIA和DWBA散射模型在整个覆盖的动量范围内,在形状和强度方面都能令人满意地再现实验动量分布,这表明扭曲波效应对于定量描述(e,2e)反应的重要性。