Baumberger F, Ingle N J C, Meevasana W, Shen K M, Lu D H, Perry R S, Mackenzie A P, Hussain Z, Singh D J, Shen Z-X
Department of Applied Physics, and Stanford Synchrotron Radiation Laboratory, Stanford University, Stanford, California 94305, USA.
Phys Rev Lett. 2006 Jun 23;96(24):246402. doi: 10.1103/PhysRevLett.96.246402. Epub 2006 Jun 20.
The electronic structure of the layered 4d transition metal oxide Sr2RhO4 is investigated by angle resolved photoemission. We find well-defined quasiparticle excitations with a highly anisotropic dispersion, suggesting a quasi-two-dimensional Fermi-liquid-like ground state. Markedly different from the isostructural Sr2RuO4, only two bands with dominant Rh 4dxz,zy character contribute to the Fermi surface. A quantitative analysis of the photoemission quasiparticle band structure is in excellent agreement with bulk data. In contrast, it is found that state-of-the-art density functional calculations in the local density approximation differ significantly from the experimental findings.
通过角分辨光电子能谱研究了层状4d过渡金属氧化物Sr2RhO4的电子结构。我们发现具有高度各向异性色散的明确定义的准粒子激发,表明存在准二维费米液体状基态。与同结构的Sr2RuO4明显不同,只有具有主导Rh 4dxz,zy特征的两个能带对费米面有贡献。光电子准粒子能带结构的定量分析与体数据非常吻合。相比之下,发现在局域密度近似下的最新密度泛函计算与实验结果有显著差异。