Welsh Gregor H, Hunt Neil T, Wynne Klaas
Department of Physics, SUPA, University of Strathclyde, Glasgow G4 0NG, Scotland, UK.
Phys Rev Lett. 2007 Jan 12;98(2):026803. doi: 10.1103/PhysRevLett.98.026803. Epub 2007 Jan 10.
The second-order processes of optical-rectification and photoconduction are well known and widely used to produce ultrafast electromagnetic pulses in the terahertz frequency domain. We present a new form of rectification that relies on the excitation of surface plasmons in metal films deposited on a shallow grating. Multiphoton ionization and ponderomotive acceleration of electrons in the enhanced evanescent field of the surface plasmons results in a femtosecond current surge and emission of terahertz electromagnetic radiation. Using gold, this rectification process is third or higher-order in the incident field.
光整流和光电导的二阶过程是众所周知的,并被广泛用于在太赫兹频域中产生超快电磁脉冲。我们提出了一种新的整流形式,它依赖于沉积在浅光栅上的金属薄膜中表面等离子体激元的激发。在表面等离子体激元增强的倏逝场中,电子的多光子电离和有质动力加速导致飞秒电流激增并发射太赫兹电磁辐射。使用金时,这种整流过程在入射场中是三阶或更高阶的。