Hurtado-Gómez Estefanía, Abián Olga, Muñoz F Javier, Hernáiz María José, Velázquez-Campoy Adrián, Neira José L
Instituto de Biología Molecular y Celular, Universidad Miguel Hernández, 03202 Elche (Alicante), Spain.
Biophys J. 2008 Aug;95(3):1336-48. doi: 10.1529/biophysj.107.126664. Epub 2008 May 2.
The bacterial PEP:sugar PTS consists of a cascade of several proteins involved in the uptake and phosphorylation of carbohydrates, and in signal transduction pathways. Its uniqueness in bacteria makes the PTS a target for new antibacterial drugs. These drugs can be obtained from peptides or protein fragments able to interfere with the first reaction of the protein cascade: the phosphorylation of the HPr by the first enzyme, the so-called enzyme EI. To that end, we designed a peptide, HPr(9-30), spanning residues 9 to 30 of the intact HPr protein, containing the active site histidine (His-15) and the first alpha-helix of HPr of Streptomyces coelicolor, HPr(sc). By using fluorescence and circular dichroism, we first determined qualitatively that HPr(sc) and HPr(9-30) did bind to EI(sc), the enzyme EI from S. coelicolor. Then, we determined quantitatively the binding affinities of HPr(9-30) and HPr(sc) for EI(sc) by using ITC and STD-NMR. The STD-NMR experiments indicate that the epitope region of HPr(9-30) was formed by residues Leu-14, His-15, Ile-21, and Val-23. The binding reaction between EI(sc) and HPr(sc) is enthalpy driven and in other species is entropy driven; further, the affinity of HPr(sc) for EI(sc) was smaller than in other species. However, the affinity of HPr(9-30) for EI(sc) was only moderately lower than that of EI(sc) for HPr(sc), suggesting that this peptide could be considered a promising hit compound for designing new inhibitors against the PTS.
糖磷酸转移酶系统(PEP:sugar PTS)由一系列参与碳水化合物摄取、磷酸化及信号转导途径的蛋白质组成。其在细菌中的独特性使磷酸转移酶系统成为新型抗菌药物的作用靶点。这些药物可从能够干扰蛋白质级联反应第一步的肽或蛋白质片段中获得:即由第一种酶(所谓的酶EI)将组氨酸蛋白(HPr)磷酸化。为此,我们设计了一种肽HPr(9 - 30),它跨越完整HPr蛋白的第9至30位残基,包含活性位点组氨酸(His - 15)以及天蓝色链霉菌HPr(HPr(sc))的第一个α - 螺旋。通过荧光和圆二色性,我们首先定性确定了HPr(sc)和HPr(9 - 30)确实与来自天蓝色链霉菌的酶EI(EI(sc))结合。然后,我们通过等温滴定量热法(ITC)和饱和转移差核磁共振(STD - NMR)定量测定了HPr(9 - 30)和HPr(sc)对EI(sc)的结合亲和力。STD - NMR实验表明,HPr(9 - 30)的表位区域由Leu - 14、His - 15、Ile - 21和Val - 23残基形成。EI(sc)与HPr(sc)之间的结合反应是由焓驱动的,而在其他物种中是由熵驱动的;此外,HPr(sc)对EI(sc)的亲和力小于其他物种。然而,HPr(9 - 30)对EI(sc)的亲和力仅略低于EI(sc)对HPr(sc)的亲和力,这表明该肽可被视为设计针对磷酸转移酶系统的新型抑制剂的有前景的先导化合物。