Weber Stefan M, Plewicki Mateusz, Weise Fabian, Lindinger Albrecht
Institut für Experimentalphysik, Freie Universität Berlin, Arnimallee 14, 14195 Berlin, Germany.
J Chem Phys. 2008 May 7;128(17):174306. doi: 10.1063/1.2907734.
We present a routine for calculating and producing customized/parametric femtosecond laser pulses for investigating molecular processes involving the polarization. It is applied on the ionization of NaK molecules by feedback-loop optimization using the recently introduced double-pass "serial setup" that is capable of phase, amplitude, and polarization modulation. The temporal subpulse encoding uses the parameters distance, intensity, zero order spectral phase, and polarization state.
我们提出了一种用于计算和生成定制/参数化飞秒激光脉冲的程序,以研究涉及极化的分子过程。该程序通过使用最近引入的能够进行相位、幅度和极化调制的双程“串联装置”,通过反馈回路优化应用于NaK分子的电离。时间子脉冲编码使用距离、强度、零阶光谱相位和极化状态等参数。