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已证明参数极化脉冲整形可用于钠钾的最优控制。

Parametric polarization pulse shaping demonstrated for optimal control of NaK.

作者信息

Weber Stefan M, Plewicki Mateusz, Weise Fabian, Lindinger Albrecht

机构信息

Institut für Experimentalphysik, Freie Universität Berlin, Arnimallee 14, 14195 Berlin, Germany.

出版信息

J Chem Phys. 2008 May 7;128(17):174306. doi: 10.1063/1.2907734.

Abstract

We present a routine for calculating and producing customized/parametric femtosecond laser pulses for investigating molecular processes involving the polarization. It is applied on the ionization of NaK molecules by feedback-loop optimization using the recently introduced double-pass "serial setup" that is capable of phase, amplitude, and polarization modulation. The temporal subpulse encoding uses the parameters distance, intensity, zero order spectral phase, and polarization state.

摘要

我们提出了一种用于计算和生成定制/参数化飞秒激光脉冲的程序,以研究涉及极化的分子过程。该程序通过使用最近引入的能够进行相位、幅度和极化调制的双程“串联装置”,通过反馈回路优化应用于NaK分子的电离。时间子脉冲编码使用距离、强度、零阶光谱相位和极化状态等参数。

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