Viswanathan Hari S, Pawar Rajesh J, Stauffer Philip H, Kaszuba John P, Carey J William, Olsen Seth C, Keating Gordon N, Kavetski Dmitri, Guthrie George D
Earth and Environmental Sciences Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA.
Environ Sci Technol. 2008 Oct 1;42(19):7280-6. doi: 10.1021/es800417x.
Sequestration of CO2 in geologic reservoirs is one of the promising technologies currently being explored to mitigate anthropogenic CO2 emissions. Large-scale deployment of geologic sequestration will require seals with a cumulative area amounting to hundreds of square kilometers per year and will require a large number of sequestration sites. We are developing a system-level model, CO2-PENS, that will predict the overall performance of sequestration systems while taking into account various processes associated with different parts of a sequestration operation, from the power plant to sequestration reservoirs to the accessible environment. The adaptability of CO2-PENS promotes application to a wide variety of sites, and its level of complexity can be increased as detailed site information becomes available. The model CO2-PENS utilizes a science-based-prediction approach by integrating information from process-level laboratory experiments, field experiments/observations, and process-level numerical modeling. The use of coupled process models in the system model of CO2-PENS provides insights into the emergent behavior of aggregate processes that could not be obtained by using individual process models. We illustrate the utility of the concept by incorporating geologic and wellbore data into a synthetic, depleted oil reservoir. In this sequestration scenario, we assess the fate of CO2 via wellbore release and resulting impacts of CO2 to a shallow aquifer and release to the atmosphere.
将二氧化碳封存于地质储层是目前正在探索的、用于减轻人为二氧化碳排放的一项很有前景的技术。大规模部署地质封存需要每年累计面积达数百平方公里的密封层,并且需要大量的封存场地。我们正在开发一个系统级模型CO2-PENS,该模型将预测封存系统的整体性能,同时考虑与封存作业不同部分相关的各种过程,从发电厂到封存储层再到可及环境。CO2-PENS的适应性促进了其在各种场地的应用,并且随着详细场地信息的获取,其复杂度可以提高。CO2-PENS模型通过整合来自过程级实验室实验、现场实验/观测以及过程级数值模拟的信息,采用基于科学预测的方法。在CO2-PENS系统模型中使用耦合过程模型,能够深入了解聚合过程的涌现行为,而这是使用单个过程模型无法获得的。我们通过将地质和井筒数据纳入一个合成的枯竭油藏来说明这一概念的实用性。在这种封存情景下,我们评估通过井筒释放的二氧化碳的归宿,以及二氧化碳对浅层含水层和向大气释放所产生的影响。