Murani A P, Severing A, Enderle M, Steffens P, Richard D
Institut Laue Langevin, 6 Rue Jules Horowitz BP 156, F-38042 Grenoble Cedex 9, France.
Phys Rev Lett. 2008 Nov 14;101(20):206405. doi: 10.1103/PhysRevLett.101.206405.
Polarized neutron scattering measurements on a single crystal of composition CeIn1Sn2 show a broad, single-ion, spectral response centered on a characteristic energy of approximately 9+/-1 meV at the zone boundary point (0 0 1.5). The zone center spectral response is closely similar in form but has a slightly reduced amplitude, smaller by some 20%. Constant-omega scans show that these intensity modulations, of amplitude approximately 10%, resembling intersite antiferromagnetic correlations, are superimposed on a mean variation that follows the Ce3+, 4f;{1}, single-ion form factor, and are tentatively attributed to q-dependent hybridization of the localized 4f state with the conduction electrons.
对组成为CeIn1Sn2的单晶进行的极化中子散射测量表明,在区边界点(0 0 1.5)处,以约9±1毫电子伏的特征能量为中心存在一个宽的单离子光谱响应。区中心的光谱响应在形式上非常相似,但幅度略有减小,减小了约20%。恒ω扫描表明,这些幅度约为10%、类似于位间反铁磁关联的强度调制叠加在一个遵循Ce3+、4f;{1}单离子形状因子的平均变化上,并初步归因于局域4f态与传导电子的q依赖杂化。