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中国南方大亚湾沉积物中多环芳烃(PAHs)的时空分布

Spatial and temporal distribution of polycyclic aromatic hydrocarbons (PAHs) in sediments from Daya Bay, South China.

作者信息

Yan Wen, Chi Jisong, Wang Zhiyuan, Huang Weixia, Zhang Gan

机构信息

CAS Key Laboratory of Marginal Sea Geology, South China Sea Institute of Oceanology, Chinese Academy of Sciences, 164 West Xingang Road, Haizhu, Guangzhou 510301, China.

出版信息

Environ Pollut. 2009 Jun;157(6):1823-30. doi: 10.1016/j.envpol.2009.01.023. Epub 2009 Feb 28.

Abstract

The spatial and temporal distribution of polycyclic aromatic hydrocarbons (PAHs) has been investigated in Daya Bay, China. The total concentration of the 16 USEPA priority PAHs in surface sediments ranged from 42.5 to 158.2 ng/g dry weight with a mean concentration of 126.2 ng/g. The spatial distribution of PAHs was site-specific and combustion processes were the main source of PAHs in the surface sediments. Total 16 priority PAH concentration in the cores 8 and 10 ranged from 77.4 to 305.7 ng/g and from 118.1 to 319.9 ng/g respectively. The variation of the 16 PAH concentrations in both cores followed the economic development in China very well and was also influenced by input pathways. Some of the PAHs were petrogenic in core 8 while pyrolytic source was dominant in core 10. In addition, pyrolytic PAHs in both cores were mainly from the coal and/or grass and wood combustion.

摘要

在中国大亚湾对多环芳烃(PAHs)的时空分布进行了调查。表层沉积物中16种美国环保署优先控制的PAHs总浓度在42.5至158.2纳克/克干重之间,平均浓度为126.2纳克/克。PAHs的空间分布具有位点特异性,燃烧过程是表层沉积物中PAHs的主要来源。岩芯8和岩芯10中16种优先PAHs的总浓度分别在77.4至305.7纳克/克和118.1至319.9纳克/克之间。两个岩芯中16种PAH浓度的变化与中国的经济发展情况高度吻合,同时也受到输入途径的影响。岩芯8中的一些PAHs具有成岩成因,而岩芯10中热解源占主导。此外,两个岩芯中的热解PAHs主要来自煤炭和/或草及木材燃烧。

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