Hahn Intaek, Brixey Laurie A, Wiener Russell W, Henkle Stacy W, Baldauf Richard
National Center for Environmental Research, U.S. Environmental Protection Agency, Washington, DC 20460, USA.
J Environ Monit. 2009 Dec;11(12):2136-45. doi: 10.1039/b907130j. Epub 2009 Oct 29.
Analyses of outdoor traffic-related particulate matter (PM) concentration distribution and fluctuation patterns in urban street canyons within a microscale distance of less than 500 m from a highway source are presented as part of the results from the Brooklyn Traffic Real-Time Ambient Pollutant Penetration and Environmental Dispersion (B-TRAPPED) study. Various patterns of spatial and temporal changes in the street canyon PM concentrations were investigated using time-series data of real-time PM concentrations measured during multiple monitoring periods. Concurrent time-series data of local street canyon wind conditions and wind data from the John F. Kennedy (JFK) International Airport National Weather Service (NWS) were used to characterize the effects of various wind conditions on the behavior of street canyon PM concentrations.Our results suggest that wind direction may strongly influence time-averaged mean PM concentration distribution patterns in near-highway urban street canyons. The rooftop-level wind speeds were found to be strongly correlated with the PM concentration fluctuation intensities in the middle sections of the street blocks. The ambient turbulence generated by shifting local wind directions (angles) showed a good correlation with the PM concentration fluctuation intensities along the entire distance of the first and second street blocks only when the wind angle standard deviations were larger than 30 degrees. Within-canyon turbulent shearing, caused by fluctuating local street canyon wind speeds, showed no correlation with PM concentration fluctuation intensities. The time-averaged mean PM concentration distribution along the longitudinal distances of the street blocks when wind direction was mostly constantly parallel to the street was found to be similar to the distribution pattern for the entire monitoring period when wind direction fluctuated wildly. Finally, we showed that two different PM concentration metrics-time-averaged mean concentration and number of concentration peaks above a certain threshold level-can possibly lead to different assessments of spatial concentration distribution patterns.
作为布鲁克林交通实时环境污染物渗透与环境扩散(B - TRAPPED)研究结果的一部分,本文呈现了对距公路源小于500米微观尺度范围内城市街道峡谷中与室外交通相关的颗粒物(PM)浓度分布及波动模式的分析。利用多个监测期内实时PM浓度的时间序列数据,研究了街道峡谷PM浓度的各种时空变化模式。同时使用当地街道峡谷风况的时间序列数据以及约翰·F·肯尼迪(JFK)国际机场国家气象局(NWS)的风数据,来描述各种风况对街道峡谷PM浓度行为的影响。我们的结果表明,风向可能会强烈影响近公路城市街道峡谷中的时间平均PM浓度分布模式。发现屋顶高度的风速与街区中部的PM浓度波动强度密切相关。仅当风向标准偏差大于30度时,当地风向(角度)变化产生的环境湍流才与第一和第二个街区整个距离上的PM浓度波动强度呈现良好的相关性。由当地街道峡谷风速波动引起的峡谷内湍流切变与PM浓度波动强度无关。当风向大多持续平行于街道时,沿街区纵向距离的时间平均PM浓度分布与风向剧烈波动时整个监测期的分布模式相似。最后,我们表明两种不同的PM浓度指标——时间平均浓度和高于某一阈值水平的浓度峰值数量——可能导致对空间浓度分布模式的不同评估。