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激光诱导近亚波长波纹的起源:表面等离激元和入射激光之间的干涉。

Origin of laser-induced near-subwavelength ripples: interference between surface plasmons and incident laser.

机构信息

Sun Yat-sen University, Guangzhou 510275, China.

出版信息

ACS Nano. 2009 Dec 22;3(12):4062-70. doi: 10.1021/nn900654v.

Abstract

We show that short-pulse laser-induced classical ripples on dielectrics, semiconductors, and conductors exhibit a prominent "non-classical" characteristic-in normal incidence the periods are definitely smaller than laser wavelengths, which indicates that the simplified scattering model should be revised. Taking into account the surface plasmons (SPs), we consider that the ripples result from the initial direct SP-laser interference and the subsequent grating-assisted SP-laser coupling. With the model, the period-decreasing phenomenon originates in the admixture of the field-distribution effect and the grating-coupling effect. Further, we propose an approach for obtaining the dielectric constant, electron density, and electron collision time of the high-excited surface. With the derived parameters, the numerical simulations are in good agreement with the experimental results. On the other hand, our results confirm that the surface irradiated by short-pulse laser with damage-threshold fluence should behave metallic, no matter for metal, semiconductor, or dielectric, and the short-pulse laser-induced subwavelength structures should be ascribed to a phenomenon of nano-optics.

摘要

我们表明,短脉冲激光在介质、半导体和导体上诱导的经典波纹表现出突出的“非经典”特征——在正入射下,周期明显小于激光波长,这表明简化的散射模型需要修正。考虑到表面等离激元(SPs),我们认为波纹是由初始的直接 SP-激光干涉和随后的光栅辅助 SP-激光耦合引起的。通过该模型,周期减小现象源于场分布效应和光栅耦合效应的混合。此外,我们提出了一种获取高激发表面介电常数、电子密度和电子碰撞时间的方法。利用得到的参数,数值模拟与实验结果吻合较好。另一方面,我们的结果证实,无论金属、半导体还是电介质,用具有损伤阈值通量的短脉冲激光辐照的表面应该表现出金属性,而短脉冲激光诱导的亚波长结构应该归因于一种纳米光学现象。

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