Liu Dong, Yan Jian-Hua, Wang Fei, Huang Qun-Xing, Chi Yong, Cen Ke-Fa
State Key Laboratory of Clean Energy Utilization, Zhejiang University, Hangzhou 310027, China.
Guang Pu Xue Yu Guang Pu Fen Xi. 2009 Dec;29(12):3185-9.
Flame soot is an import product as a result of incomplete combustion of hydrocarbon fuels, and has important effect on the generation of some pollutant. The optical properties of the soot are the base for the optical combustion diagnostics. Terahertz time-domain spectroscopy technique was used to study the optical properties of the soot within 0.2-1.6 THz and the frequency-domain spectra were obtained through Fourier transform. The complex refractive index of the soot was deduced by the fixed-point iteration. The comparison of the complex refractive index between terahertz spectra domain and thermal radiation spectra domain was conducted and two methods of extracting the parameters were also compared. The results indicated that the soot has strong absorption in the studied spectra and the difference in the refractive index between the two spectra domains was not obvious, but the absorptive index variation in the thermal radiation spectra domain was larger. The difference between the two parameter extraction methods was not significant. The deduced results can provide the optical data of soot for the application of terahertz time-domain spectroscopy technique to the optical combustion diagnostics, and extend the optical combustion diagnostics application area.
火焰烟灰是碳氢化合物燃料不完全燃烧的一种重要产物,并且对某些污染物的生成有重要影响。烟灰的光学特性是光学燃烧诊断的基础。利用太赫兹时域光谱技术研究了0.2 - 1.6太赫兹范围内烟灰的光学特性,并通过傅里叶变换获得了频域光谱。通过定点迭代法推导了烟灰的复折射率。对太赫兹光谱域和热辐射光谱域的复折射率进行了比较,还比较了两种参数提取方法。结果表明,烟灰在所研究的光谱范围内有较强的吸收,两个光谱域的折射率差异不明显,但热辐射光谱域的吸收指数变化较大。两种参数提取方法的差异不显著。推导结果可为太赫兹时域光谱技术应用于光学燃烧诊断提供烟灰的光学数据,并扩展光学燃烧诊断的应用领域。