Physics Department, Kent State University, Kent, Ohio 44242, USA.
Phys Rev Lett. 2010 Feb 12;104(6):066402. doi: 10.1103/PhysRevLett.104.066402. Epub 2010 Feb 9.
We present magnetization (M) data of the d-metal alloy Ni(1-x)V(x) at vanadium concentrations close to x(c) approximately = 11.4% where the onset of long-range ferromagnetic (FM) order is suppressed to zero temperature. Above x(c), the temperature (T) and magnetic field (H) dependencies of the magnetization are best described by simple nonuniversal power laws. The exponents of M/H approximately T(-gamma) and M approximately H(alpha) are related by 1-gamma = alpha for wide temperature (10 < T < or = 300 K) and field (H < or = 5 T) ranges. gamma is strongly x dependent, decreasing from 1 at x approximately = x(c) to gamma < 0.1 for x = 15%. This behavior is not compatible with either classical or quantum critical behavior in a clean 3D FM. Instead it closely follows the predictions for a quantum Griffiths phase associated with a quantum phase transition in a disordered metal. Deviations at the lowest temperatures hint at a freezing of large clusters and the onset of a cluster glass phase.
我们呈现了 d 族金属合金 Ni(1-x)V(x)在接近 x(c)约等于 11.4%的钒浓度下的磁化率 (M) 数据,此时长程铁磁 (FM) 有序被抑制到零温度。在 x(c)以上,磁化率随温度 (T) 和磁场 (H) 的依赖关系最好用简单的非普适幂律来描述。M/H 大约 T(-gamma)和 M 大约 H(alpha)的指数通过 1-gamma = alpha 相关,适用范围很广,温度为 10 < T < or = 300 K,磁场为 H < or = 5 T。gamma 强烈依赖于 x,从 x 大约等于 x(c)时的 1 减小到 x = 15%时的 gamma < 0.1。这种行为与清洁 3D FM 中的经典或量子临界行为都不兼容。相反,它与与无序金属中的量子相变相关的量子 Griffiths 相位的预测密切相关。在最低温度下的偏差暗示着大团簇的冻结和团簇玻璃相的开始。