Department of Physics, Worcester Polytechnic Institute, 100 Institute Road, Worcester, Massachusetts 01609, USA.
J Chem Phys. 2010 May 7;132(17):174701. doi: 10.1063/1.3374437.
Capillary waves have been observed in systems ranging from the surfaces of ordinary fluids to interfaces in biological membranes and have been one of the most studied areas in the physics of fluids. Recent advances in fluorescence microscopy and imaging enabled quantitative measurements of thermally driven capillary waves in lipid monolayers and bilayers, which resulted in accurate measurements of the line tension in monolayer domains. Even though there has been a considerable amount of work on the statics and dynamics of capillary waves in three dimensions, to the best of our knowledge, there is no detailed theoretical analysis for two-dimensional droplet morphologies. In this paper, we derive the dynamic correlation function for two-dimensional fluid droplets using linear response theory and verify our results using a novel particle-based simulation technique for binary mixtures.
已经在从普通流体表面到生物膜界面等各种系统中观察到毛细波,并且它一直是流体物理学中研究最多的领域之一。荧光显微镜和成像技术的最新进展使我们能够对脂质单层和双层中的热驱动毛细波进行定量测量,从而可以准确测量单层域中的线张力。尽管已经有相当多的关于三维毛细波的静态和动态的工作,但据我们所知,对于二维液滴形态还没有详细的理论分析。在本文中,我们使用线性响应理论推导出二维流体液滴的动态相关函数,并使用二元混合物的新型基于粒子的模拟技术验证我们的结果。