Department of Physics, Florida State University, Tallahassee, FL 32306, USA.
J Phys Condens Matter. 2011 Apr 27;23(16):164203. doi: 10.1088/0953-8984/23/16/164203. Epub 2011 Apr 6.
The low temperature behaviour of single crystalline SrHo(2)O(4) has been characterized by dc magnetic susceptibility, heat capacity, and neutron scattering experiments. Our results show that despite the lack of magnetic long-ranged ordering in the presence of strong antiferromagnetic correlations, SrHo(2)O(4) does not order down to 1.8 K. Elastic neutron scattering experiments show prominent magnetic diffuse scattering correlated with a broad feature in the dc susceptibility at T = 4 K, indicative of magnetic short-ranged ordering of the Ho(3) spins. Inelastic neutron scattering shows the presence of five crystal field levels up to 80 K in energy, in agreement with the integration of the magnetic specific heat component yielding Rln5 entropy release. The magnetic short-ranged ordering is fitted to a nearest neighbour interaction model with good agreement.
单晶 SrHo(2)O(4)的低温行为已通过直流磁化率、比热和中子散射实验进行了表征。我们的结果表明,尽管存在强烈的反铁磁关联,但 SrHo(2)O(4)在 1.8 K 以下没有出现磁长程有序。弹性中子散射实验表明,在 T = 4 K 时,与直流磁化率中的宽特征相关的磁弥散散射显著,表明 Ho(3)自旋的磁短程有序。非弹性中子散射表明,在能量高达 80 K 的范围内存在五个晶场能级,与磁比热分量的积分一致,产生 Rln5 熵释放。磁短程有序用良好吻合的最近邻相互作用模型进行拟合。