LARA - Laboratório de Radioecologia, Instituto de Física, Universidade Federal Fluminense, Av. Gal Milton Tavares de Souza, s/no, Gragoatá, 24210-340 Niterói, RJ, Brazil.
J Environ Radioact. 2011 Nov;102(11):1055-61. doi: 10.1016/j.jenvrad.2011.06.001. Epub 2011 Jul 5.
Health hazard from natural radioactivity in Brazilian granites, covering the walls and floor in a typical dwelling room, was assessed by indirect methods to predict external gamma-ray dose rates and radon concentrations. The gamma-ray dose rate was estimated by a Monte Carlo simulation method and validated by in-situ measurements with a NaI spectrometer. Activity concentrations of (232)Th, (226)Ra, and (40)K in an extensive selection of Brazilian commercial granite samples measured by using gamma-ray spectrometry were found to be 4.5-450 Bq kg(-1), 4.9-160 Bq kg(-1) and 190-2029 Bq kg(-1), respectively. The maximum external gamma-ray dose rate from floor and walls covered with the Brazilian granites in the typical dwelling room (5.0 m × 4.0 m area, 2.8 m height) was found to be 120 nGy h(-1), which is comparable with the average worldwide exposure to external terrestrial radiation of 80 nGy h(-1) due to natural sources, proposed by United Nations Scientific Committee on the Effects of Atomic Radiation. Radon concentrations in the room were also estimated by a simple mass balance equation and exhalation rates calculated from the measured values of (226)Ra concentrations and the material properties. The results showed that the radon concentration in the room ventilated adequately (0.5 h(-1)) will be lower than 100 Bq m(-3), value recommended as a reference level by the World Health Organization.
采用间接方法评估了巴西花岗岩(用于覆盖典型居住房间的墙壁和地板)中的天然放射性对健康的危害,以预测外照射γ射线剂量率和氡浓度。采用蒙特卡罗模拟方法估算γ射线剂量率,并通过使用 NaI 谱仪进行现场测量进行验证。使用γ射线光谱法测量了广泛选择的巴西商业花岗岩样品中的 (232)Th、(226)Ra 和 (40)K 的活度浓度,结果分别为 4.5-450 Bq kg(-1)、4.9-160 Bq kg(-1) 和 190-2029 Bq kg(-1)。在典型居住房间(5.0 m×4.0 m 面积,2.8 m 高)中用巴西花岗岩覆盖地板和墙壁时的最大外照射γ射线剂量率为 120 nGy h(-1),这与联合国原子辐射效应科学委员会建议的由于天然来源而导致的全球平均外照射陆地辐射 80 nGy h(-1)相当。还通过简单的质量平衡方程估算了房间内的氡浓度,并根据测量的 (226)Ra 浓度值和材料特性计算了氡的释放率。结果表明,在充分通风的房间(0.5 h(-1)) 中,氡浓度将低于 100 Bq m(-3),世界卫生组织建议将其作为参考水平。