Zhu Xiangde, Sun Yuping, Zhang Shuhua, Wang Jianglong, Zou Liangjian, Delong Lance E, Zhu Xuebin, Luo Xuan, Wang Bosen, Li Gang, Yang Zhaorong, Song Wenhai
Key Laboratory of Materials Physics, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei 230031, People's Republic of China.
J Phys Condens Matter. 2009 Apr 8;21(14):145701. doi: 10.1088/0953-8984/21/14/145701. Epub 2009 Mar 5.
The anisotropic superconducting state properties in Cu(0.03)TaS(2) have been investigated by magnetization, magnetoresistance and specific heat measurements. They clearly show that Cu(0.03)TaS(2) undergoes a superconducting transition at T(C) = 4.03 K. The obtained superconducting parameters demonstrate that Cu(0.03)TaS(2) is an anisotropic type-II superconductor. Combining specific heat jump ΔC/γ(n)T(C) = 1.6(4), gap ratio 2Δ/k(B)T(C) = 4.0(9) and the estimated electron-phonon coupling constant λ∼0.68, the superconductivity in Cu(0.03)TaS(2) is explained within the intermediate coupling BCS scenario. First-principles electronic structure calculations suggest that copper intercalation of 2H-TaS(2) causes a considerable increase of the Fermi surface volume and the carrier density, which suppresses the CDW fluctuation and favors the raise of T(C).
通过磁化、磁阻和比热测量研究了Cu(0.03)TaS(2)中的各向异性超导态特性。结果清楚地表明,Cu(0.03)TaS(2)在T(C)=4.03 K时发生超导转变。所获得的超导参数表明Cu(0.03)TaS(2)是一种各向异性的II型超导体。结合比热跃变ΔC/γ(n)T(C)=1.6(4)、能隙比2Δ/k(B)T(C)=4.0(9)以及估计的电子-声子耦合常数λ∼0.68,Cu(0.03)TaS(2)中的超导性可在中间耦合BCS理论框架内得到解释。第一性原理电子结构计算表明,2H-TaS(2)中铜的嵌入导致费米面体积和载流子密度显著增加,这抑制了电荷密度波涨落并有利于T(C)的升高。