INM-Leibniz Institut für Neue Materialien, Campus D2 2, 66123, Saarbrücken, Germany.
Phys Rev Lett. 2011 Sep 30;107(14):144303. doi: 10.1103/PhysRevLett.107.144303.
Nanometer-scale friction measurements on a Au(111) surface have been performed at temperatures between 30 and 300 K by means of atomic force microscopy. Stable stick slip with atomic periodicity is observed at all temperatures, showing only weak dependence on temperature between 300 and 170 K. Below 170 K, friction increases with time and a distortion of the stick-slip characteristic is observed. Low friction and periodic stick slip can be reestablished by pulling the tip out of contact and subsequently restoring the contact. A comparison with molecular dynamics simulations indicates that plastic deformation within a growing gold junction leads to the observed frictional behavior at low temperatures. The regular stick slip with atomic periodicity observed at room temperature is the result of a dynamic equilibrium shape of the contact, as microscopic wear damage is observed to heal in the sliding contact.
采用原子力显微镜在 30 至 300 K 的温度范围内对 Au(111)表面进行了纳米级摩擦测量。在所有温度下均观察到稳定的具有原子周期性的黏滑,仅在 300 至 170 K 之间表现出对温度的微弱依赖性。在 170 K 以下,摩擦力随时间增加,并且观察到黏滑特性的变形。通过将尖端拉出接触并随后恢复接触,可以重新建立低摩擦和周期性黏滑。与分子动力学模拟的比较表明,在生长的金结内的塑性变形导致了低温下观察到的摩擦行为。在室温下观察到的具有原子周期性的规则黏滑是接触的动态平衡形状的结果,因为在滑动接触中观察到微观磨损损伤得到了修复。