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毫开尔文温度下顺磁电子自旋的磁共振力显微镜。

Magnetic resonance force microscopy of paramagnetic electron spins at millikelvin temperatures.

机构信息

Leiden Institute of Physics, Leiden University, Niels Bohrweg 2, 2333CA, Leiden, The Netherlands.

出版信息

Nat Commun. 2011 Dec 6;2:572. doi: 10.1038/ncomms1581.

Abstract

Magnetic resonance force microscopy (MRFM) is a powerful technique to detect a small number of spins that relies on force detection by an ultrasoft magnetically tipped cantilever and selective magnetic resonance manipulation of the spins. MRFM would greatly benefit from ultralow temperature operation, because of lower thermomechanical noise and increased thermal spin polarization. Here we demonstrate MRFM operation at temperatures as low as 30 mK, thanks to a recently developed superconducting quantum interference device (SQUID)-based cantilever detection technique, which avoids cantilever overheating. In our experiment, we detect dangling bond paramagnetic centres on a silicon surface down to millikelvin temperatures. Fluctuations of such defects are supposedly linked to 1/f magnetic noise and decoherence in SQUIDs, as well as in several superconducting and single spin qubits. We find evidence that spin diffusion has a key role in the low-temperature spin dynamics.

摘要

磁共振力显微镜(MRFM)是一种强大的技术,可用于检测少量的自旋,其依赖于超软磁尖端悬臂的力检测以及自旋的选择性磁共振操纵。由于更低的热机械噪声和增加的热自旋极化,MRFM 将极大地受益于超低温度操作。在这里,我们展示了在低至 30mK 的温度下进行的 MRFM 操作,这要归功于最近开发的基于超导量子干涉器件(SQUID)的悬臂检测技术,该技术避免了悬臂过热。在我们的实验中,我们在毫开尔文温度下检测到硅表面上的悬空键顺磁中心。据推测,这种缺陷的波动与 SQUIDs 以及几种超导和单自旋量子位中的 1/f 磁噪声和退相干有关。我们发现有证据表明,自旋扩散在低温自旋动力学中起着关键作用。

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