Cui Weicheng, Qi Shuibao, Chen Weizhong, Zhou Chao, Tu Juan
The Key Laboratory of Modern Acoustics, Ministry of Education, Institute of Acoustics, Nanjing University, Nanjing 210093, China.
Phys Rev E Stat Nonlin Soft Matter Phys. 2012 Feb;85(2 Pt 2):026304. doi: 10.1103/PhysRevE.85.026304. Epub 2012 Feb 7.
The driving parametric regions in frequency-amplitude space and the optimal parameters for single-bubble sonoluminescence (SBSL) in alcohol aqueous solutions are studied systematically by taking measurements of the spectrum and bubble dynamics. The experimental results show that with an increase in alcohol concentration, the region shrinks and shifts. The optimized parameters differ for alcohol solutions having different concentrations, and SBSL driven by fixed parameters dims quickly and is even destroyed immediately with the addition of a small amount of alcohol to pure water. Furthermore, it is seen that the intensity of optimized SBSL decreases as the alcohol concentration increases. The corresponding measurements of the dynamics of the optimized SBSL bubble show that the maximum bubble radius at an alcohol concentration of 1.04 mM is only half that for pure water. Meanwhile, the optimized driving amplitude acquired by direct measurement and that obtained by fitting the radius-time curves with the Rayleigh-Plesset equation both decrease by 12% in the same comparison. Therefore, a decrease in the driving acoustic pressure may be an important reason for the decrease in the optimized SBSL intensity, which should help clarify SBSL mechanisms in alcohol aqueous solutions.
通过对光谱和气泡动力学进行测量,系统地研究了乙醇水溶液中频率 - 振幅空间内的驱动参数区域以及单泡声致发光(SBSL)的最佳参数。实验结果表明,随着乙醇浓度的增加,该区域会缩小并发生偏移。不同浓度乙醇溶液的优化参数不同,向纯水中添加少量乙醇后,固定参数驱动的SBSL会迅速变暗甚至立即被破坏。此外,可以看出优化后的SBSL强度随着乙醇浓度的增加而降低。对优化后的SBSL气泡动力学进行的相应测量表明,乙醇浓度为1.04 mM时的最大气泡半径仅为纯水时的一半。同时,在相同比较中,通过直接测量获得的优化驱动振幅以及通过用瑞利 - 普莱斯方程拟合半径 - 时间曲线得到的驱动振幅均下降了12%。因此,驱动声压的降低可能是优化后的SBSL强度降低的一个重要原因,这有助于阐明乙醇水溶液中的SBSL机制。