Surface Science Research Centre and Department of Physics, The University of Liverpool, Liverpool L69 3BX, UK.
Philos Trans A Math Phys Eng Sci. 2012 Jun 28;370(1969):2930-48. doi: 10.1098/rsta.2011.0220.
If crystal structures can be viewed as repositories of information, then crystal surfaces offer a pathway by which this information can be used to grow new structures through the process of epitaxy. The information transfer process is one of self-organization, and the kinetic and energetic factors influencing this are complex. They include the relative strengths of the adsorbate-adsorbate and adsorbate-substrate interactions, the flux of incoming species and the temperature of the system. In this brief review, we explore how the interplay of these factors influences the degree to which the epitaxial structures retain the 'memory' of the template, illustrating the discussion with examples from epitaxy on quasi-crystal surfaces.
如果晶体结构可以被视为信息的存储库,那么晶体表面提供了一种途径,可以通过外延生长过程利用这些信息来生长新的结构。信息传递过程是一个自组织的过程,影响这一过程的动力学和能量因素很复杂。它们包括吸附质-吸附质和吸附质-衬底相互作用的相对强度、入射物种的通量以及系统的温度。在这篇简要的综述中,我们探讨了这些因素的相互作用如何影响外延结构保留模板“记忆”的程度,并通过在准晶表面外延的例子来说明讨论。