McCrillis R C, Burnet P G
Air and Energy Engineering Research Laboratory, U.S. Environmental Protection Agency Research Triangle Park, North Carolina 27711.
Toxicol Ind Health. 1990 Oct;6(5):95-102.
During the winter of 1986-87, the U.S. Environmental Protection Agency (EPA) conducted an emission measurement program in Boise, ID, as part of the Integrated Air Cancer Project (IACP). This program was designed to identify the potential mutagenic impact of residential wood burning on ambient and indoor air. One facet of this field sampling effort involved obtaining emission samples from chimneys serving wood burning appliances in Boise. As a companion to the field source sampling, a parallel project was undertaken in an instrumented woodstove test laboratory to quantify woodstove emissions during operations typical of Boise usage. Two woodstoves were operated in a test laboratory over a range of burnrates, burning either eastern oak or white pine from the Boise, ID, area. A conventional stove, manufactured in the Boise area, was tested at altitudes of 90 and 825 m. A catalytic stove was tested only at the high altitude facility. All emission tests were started with kindling a fire in a cold stove using black and white newsprint. Emissions were collected using the wood stove dilution sampling system (WSDSS) for a continuous period of about 8 hours, encompassing start-up and several wood additions. The results showed wide variability probably due primarily to the difficulty in duplicating conditions during start-up. Total WSDSS emissions showed the expected inverse correlations with burnrate for the conventional stove and nearly flat for the catalytic stove. While there appeared to be little or no correlation of total WSDSS emissions with altitude, the sum of the 16 polynuclear aromatic hydrocarbons (PAHs) quantified showed an inverse correlation with altitude: higher PAH emissions at the lower altitude.
1986 - 1987年冬季,作为综合空气癌症项目(IACP)的一部分,美国环境保护局(EPA)在爱达荷州博伊西市开展了一项排放测量项目。该项目旨在确定居民燃木对室外和室内空气潜在的致突变影响。这项实地采样工作的一个方面涉及从博伊西市为燃木器具服务的烟囱中获取排放样本。作为实地源采样的补充,在一个配备仪器的燃木炉灶测试实验室开展了一个平行项目,以量化在博伊西市典型使用情况下运行期间的燃木炉灶排放。在一个测试实验室中,两台燃木炉灶在一系列燃烧速率下运行,燃烧的是来自爱达荷州博伊西市地区的东部橡木或白松。一台在博伊西市地区制造的传统炉灶在海拔90米和825米处进行了测试。一台催化炉灶仅在高海拔设施进行了测试。所有排放测试都是在冷炉灶中使用黑白新闻纸生火开始的。使用燃木炉灶稀释采样系统(WSDSS)连续约8小时收集排放物,包括启动阶段和多次添加木材的过程。结果显示差异很大,这可能主要是由于在启动阶段难以复制条件。传统炉灶的WSDSS总排放量与燃烧速率呈现预期的负相关,而催化炉灶的几乎持平。虽然WSDSS总排放量与海拔似乎几乎没有相关性,但定量的16种多环芳烃(PAHs)的总和与海拔呈现负相关:海拔较低时PAH排放量较高。